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不含扩散和热传递的含金属单体聚合的行波

Traveling-waves of metal-containing monomer polymerization without diffusion and heat-transfer.

作者信息

Zakiev S E, Shershnev V A, Yadav B C, Kvurt Yu P, Dzhardimalieva G I

机构信息

Institute of Problems of Chemical Physics, RAS, Chernogolovka, Moscow Region, Russia.

Babasaheb Bhimrao Ambedkar University, Lucknow- 226025, U.P., India.

出版信息

Heliyon. 2019 Nov 16;5(11):e02829. doi: 10.1016/j.heliyon.2019.e02829. eCollection 2019 Nov.

DOI:10.1016/j.heliyon.2019.e02829
PMID:31763482
原文链接:https://pmc.ncbi.nlm.nih.gov/articles/PMC6861569/
Abstract

The new approach for modeling kinetics of complex spatial self-propagating traveling-wave reactions is proposed. This approach is intended to replace well-known reaction-diffusion equations and self-propagating high-temperature synthesis (SHS) as methods for mathematical modeling of spatial propagation of chemical reactions. A chemical kinetic model for frontal polymerization of metal-containing monomers under this approach is suggested.

摘要

提出了一种用于对复杂空间自传播行波反应动力学进行建模的新方法。该方法旨在取代著名的反应扩散方程和自蔓延高温合成法（SHS），作为化学反应空间传播数学建模的方法。在此方法下，提出了一种含金属单体前沿聚合的化学动力学模型。

https://cdn.ncbi.nlm.nih.gov/pmc/blobs/8811/6861569/e1d857ea7659/gr3.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/8811/6861569/37bf20698383/gr1.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/8811/6861569/35b5a8e98a3c/gr2.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/8811/6861569/e1d857ea7659/gr3.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/8811/6861569/37bf20698383/gr1.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/8811/6861569/35b5a8e98a3c/gr2.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/8811/6861569/e1d857ea7659/gr3.jpg

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本文引用的文献

1
Frontal Polymerization of Dicyclopentadiene: A Numerical Study.双环戊二烯的前沿聚合：数值研究
J Phys Chem B. 2018 Apr 26;122(16):4583-4591. doi: 10.1021/acs.jpcb.7b12316. Epub 2018 Apr 17.