Liu Yu, Vaitiekėnas Saulius, Martí-Sánchez Sara, Koch Christian, Hart Sean, Cui Zheng, Kanne Thomas, Khan Sabbir A, Tanta Rawa, Upadhyay Shivendra, Cachaza Martin Espiñeira, Marcus Charles M, Arbiol Jordi, Moler Kathryn A, Krogstrup Peter
Microsoft Quantum Materials Lab Copenhagen , 2800 Lyngby , Denmark.
Center for Quantum Devices, Niels Bohr Institute , University of Copenhagen , 2100 Copenhagen , Denmark.
Nano Lett. 2020 Jan 8;20(1):456-462. doi: 10.1021/acs.nanolett.9b04187. Epub 2019 Dec 3.
Nanowires can serve as flexible substrates for hybrid epitaxial growth on selected facets, allowing for the design of heterostructures with complex material combinations and geometries. In this work we report on hybrid epitaxy of freestanding vapor-liquid-solid grown and in-plane selective area grown semiconductor-ferromagnetic insulator-superconductor (InAs/EuS/Al) nanowire heterostructures. We study the crystal growth and complex epitaxial matching of wurtzite and zinc-blende InAs/rock-salt EuS interfaces as well as rock-salt EuS/face-centered cubic Al interfaces. Because of the magnetic anisotropy originating from the nanowire shape, the magnetic structure of the EuS phase is easily tuned into single magnetic domains. This effect efficiently ejects the stray field lines along the nanowires. With tunnel spectroscopy measurements of the density of states, we show that the material has a hard induced superconducting gap, and magnetic hysteretic evolution which indicates that the magnetic exchange fields are not negligible. These hybrid nanowires fulfill key material requirements for serving as a platform for spin-based quantum applications, such as scalable topological quantum computing.
纳米线可作为在特定晶面上进行混合外延生长的柔性衬底,从而实现具有复杂材料组合和几何形状的异质结构设计。在本工作中,我们报道了独立生长的气-液-固生长和面内选择性区域生长的半导体-铁磁绝缘体-超导体(InAs/EuS/Al)纳米线异质结构的混合外延。我们研究了纤锌矿型和闪锌矿型InAs/岩盐型EuS界面以及岩盐型EuS/面心立方Al界面的晶体生长和复杂外延匹配。由于纳米线形状产生的磁各向异性,EuS相的磁结构很容易被调制成单磁畴。这种效应有效地将杂散场线沿纳米线方向射出。通过对态密度的隧道光谱测量,我们表明该材料具有硬诱导超导能隙以及磁滞演化,这表明磁交换场不可忽略。这些混合纳米线满足了作为基于自旋的量子应用平台(如可扩展拓扑量子计算)的关键材料要求。