Cao Lianzhen, Liu Xia, Guo Zhen, Zhou Lianqun
Department of Physics and Optoelectronic Engineering, Weifang University, Weifang 261061, China.
CASKey Lab of Bio-Medical Diagnostics, Suzhou Institute of Biomedical Engineering and Technology, Chinese Academy of Sciences, Suzhou 215163, China.
Micromachines (Basel). 2019 Nov 27;10(12):821. doi: 10.3390/mi10120821.
With the rise of nanoscience and nanotechnologies, especially the continuous deepening of research on low-dimensional materials and structures, various kinds of light-emitting devices based on nanometer-structured materials are gradually becoming the natural candidates for the next generation of advanced optoelectronic devices with improved performance through engineering their interface/surface properties. As dimensions of light-emitting devices are scaled down to the nanoscale, the plentitude of their surface/interface properties is one of the key factors for their dominating device performance. In this paper, firstly, the generation, classification, and influence of surface/interface states on nanometer optical devices will be given theoretically. Secondly, the relationship between the surface/interface properties and light-emitting diode device performance will be investigated, and the related physical mechanisms will be revealed by introducing classic examples. Especially, how to improve the performance of light-emitting diodes by using factors such as the surface/interface purification, quantum dots (QDs)-emitting layer, surface ligands, optimization of device architecture, and so on will be summarized. Finally, we explore the main influencing actors of research breakthroughs related to the surface/interface properties on the current and future applications for nanostructured light-emitting devices.
随着纳米科学和纳米技术的兴起,特别是对低维材料和结构研究的不断深入,基于纳米结构材料的各种发光器件正逐渐成为下一代先进光电器件的自然候选者,通过设计其界面/表面特性可提高器件性能。随着发光器件的尺寸缩小到纳米尺度,其丰富的表面/界面特性是决定器件性能的关键因素之一。本文首先从理论上阐述纳米光学器件表面/界面态的产生、分类及其影响。其次,研究表面/界面特性与发光二极管器件性能之间的关系,并通过引入经典实例揭示相关物理机制。特别地,将总结如何利用表面/界面净化、量子点(QDs)发光层、表面配体、器件结构优化等因素来提高发光二极管的性能。最后,我们探讨与表面/界面特性相关的研究突破对纳米结构发光器件当前和未来应用的主要影响因素。