Miguet Jonas, Pasquet Marina, Rouyer Florence, Fang Yuan, Rio Emmanuelle
Laboratoire de Physique des Solides, CNRS, Université Paris-Saclay, 91405 Orsay, France.
Université Paris-Est, Laboratoire Navier (UMR 8205 CNRS, ENPC ParisTech, IFSTTAR), 5 boulevard Descartes, 77 454 Champs-Sur-Marne, France.
Soft Matter. 2020 Jan 28;16(4):1082-1090. doi: 10.1039/c9sm01490j. Epub 2019 Dec 23.
Surface bubbles have attracted much interest in the past few decades. In this article, we aim to explore the lifetime and thinning dynamics of centimetric surface bubbles. We study the impact of the bubble size as well as that of the atmospheric humidity through a careful control and systematic variation of the relative humidity in the measuring chamber. We first address the question of the drainage under saturated water vapor conditions and show that a model including both capillary and gravity driven drainage provides the best prediction for this process. Additionally, unprecedented statistics on the bubble lifetimes confirm experimentally that this parameter is set by evaporation to leading order. We make use of a model based on the overall thinning dynamics of the thin film and assume a rupture thickness of the order 10-100 nm to obtain a good representation of these data. For experiments conducted far from saturation, the convective evaporation of the bath is shown to dominate the overall mass loss in the cap film due to evaporation.
在过去几十年中,表面气泡引起了人们的广泛关注。在本文中,我们旨在探究厘米级表面气泡的寿命和变薄动力学。我们通过仔细控制和系统改变测量室中的相对湿度,研究了气泡大小以及大气湿度的影响。我们首先解决饱和水蒸气条件下的排水问题,并表明一个同时包含毛细管和重力驱动排水的模型能对这一过程提供最佳预测。此外,关于气泡寿命的前所未有的统计数据通过实验证实,该参数主要由蒸发决定。我们利用一个基于薄膜整体变薄动力学的模型,并假设破裂厚度在10 - 100纳米量级,从而很好地呈现了这些数据。对于在远离饱和状态下进行的实验,浴液的对流蒸发被证明在盖膜因蒸发导致的总质量损失中占主导地位。