Chen Rui, Li Yongjun, Yang Haixia, Fan Yufang
Gansu Provincial Center for Disease Control and Prevention, Lanzhou 730000, China.
Wei Sheng Yan Jiu. 2019 Nov;48(6):957-963.
To understand the pollution level of polycyclic aromatic hydrocarbons(PAHs) in community fine particulate matter(PM_(2. 5)) in Lanzhou community, and assess the risk of cancer.
Samples of atmospheric fine particles were collected in communities A and B of Lanzhou City from 10 to 16 of each month in 2018. The mass concentration and composition of 16 kinds of optimal control to the EPA PAHs, such as naphthalene(Nap), acenaphthylene(Acy), philippines(Phe), acenaphthene(Ace), fluorene(FI), anthracene(Ant), fluoranthene(Flu), pyrene(Pyr), chrysene(Chr), benzo(a) anthracene(BaA), benzene(b) fluoranthracene(BbF), benzene(k) fluoranthracene(BkF), benzo(a) pyrene(BaP), dibenzene(a, h) anthracene(DahA), benzene(g, h, i) perylene(BghiP) and indene(1, 2, 3-cd)pyrene(IcdP), were analysed, and the toxicity were assessed by toxicity equivalent concentration and lifetime excess carcinogenic risk(ECR).
The annual average PM_(2. 5) concentrations in community A and B were 70 μg/m3, 2 times the national standard. The average annual PAHs concentrations in community A and B were 113. 56(5. 22-485. 71) and 55. 68(2. 39-257. 43) ng/m3, respectively. In addition, in winter, spring and autumn, the PAHs of the two communities were mainly 3-5 rings, 3-ring and 6-ring PAHs were the main components in summer. The result of feature ratio method were shown that BaP of 16 kinds of PAHs was the equivalent mass concentration(BaPeq) range of 0. 00017-3. 19 ng/m3, ΣBaPeqin community A and B were 7. 64 and5. 11 ng/m3, respectively. BaP and DahA were the most toxic, All of them contributed more than 70% to ΣBaPeq, the total ECR of Σ16 PAHs in community A and B were 6. 64×10(-4) and 4. 44×10~(-4), respectivel.
BaP and DahA have certain potential health risks to residents in communities a and B of Lanzhou.
了解兰州市社区细颗粒物(PM₂.₅)中多环芳烃(PAHs)的污染水平,并评估其致癌风险。
于2018年每月10日至16日在兰州市A、B两个社区采集大气细颗粒物样本。分析了美国环境保护局(EPA)优先控制的16种多环芳烃的质量浓度和组成,如萘(Nap)、苊烯(Acy)、菲(Phe)、苊(Ace)、芴(FI)、蒽(Ant)、荧蒽(Flu)、芘(Pyr)、 Chrysene(Chr)、苯并(a)蒽(BaA)、苯并(b)荧蒽(BbF)、苯并(k)荧蒽(BkF)、苯并(a)芘(BaP)、二苯并(a,h)蒽(DahA)、苯并(g,h,i)苝(BghiP)和茚并(1,2,3-cd)芘(IcdP),并通过毒性当量浓度和终生超额致癌风险(ECR)评估其毒性。
A、B两个社区的PM₂.₅年均浓度分别为70μg/m³,是国家标准的2倍。A、B两个社区的PAHs年均浓度分别为113.56(5.22 - 485.71)和55.68(2.39 - 257.43)ng/m³。此外,冬季、春季和秋季,两个社区的PAHs主要为3 - 5环,夏季以3环和6环PAHs为主。特征比值法结果显示,16种PAHs中BaP的等效质量浓度(BaPeq)范围为0.00017 - 3.19ng/m³,A、B两个社区的ΣBaPeq分别为7.64和5.11ng/m³。BaP和DahA毒性最强,它们对ΣBaPeq的贡献率均超过70%,A、B两个社区Σ16种PAHs的总ECR分别为6.64×10⁻⁴和4.44×10⁻⁴。
BaP和DahA对兰州市A、B两个社区居民具有一定的潜在健康风险。