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中国北方典型浅水湖中汞的分布及其从沉积物中的再释放。

Mercury distribution in a typical shallow lake in northern China and its re-emission from sediment.

机构信息

School of Water Conservancy and Environment, University of Jinan, Jinan, 250022, China.

State Key Laboratory of Environmental Geochemistry, Institute of Geochemistry, Chinese Academy of Sciences, Guiyang, 550081, China; University of Chinese Academy of Sciences, Beijing, 100049, China.

出版信息

Ecotoxicol Environ Saf. 2020 Apr 1;192:110316. doi: 10.1016/j.ecoenv.2020.110316. Epub 2020 Feb 13.

Abstract

Mercury (Hg) re-emission from sediment is an important process in the biogeochemistry cycles of Hg in the aquatic ecosystem. The contribution of Hg released from sediment to water remains unclear for some shallow lakes. Lake Nansi is a typical shallow lake in northern China that is divided into upper and lower lakes by a dam. The Hg species in the water profile and sediment were measured from two sampling sites in the lake. Nansi Lake was not markedly contaminated by Hg. The Hg profile in the sediment indicated that the demand for energy and the policy management in the catchment influenced the Hg accumulation in its sediment. On the basis of Fick's first law and the sedimentation rate, the diffusion flux of dissolved Hg from sediment to overlying water and the accumulation flux were estimated. According to one-year scale estimation, approximately 10%-13% the Hg in the sediments can be re-released into the overlying water. The Hg diffused from the sediment accounted for 7.9%-16% of the Hg in the overlying water. These results of this study improve the understanding of the sources of pollution in water and enable researchers to focus on the contribution of sediment to the pollution of water in shallow lakes.

摘要

汞(Hg)从沉积物中的再释放是水生生态系统中汞生物地球化学循环的一个重要过程。对于一些浅水湖泊,从沉积物中释放到水中的汞的贡献仍不清楚。南四湖是中国北方的一个典型浅水湖,由一个大坝将其分为上湖和下湖。对来自湖中两个采样点的水剖面和沉积物中的汞形态进行了测量。南四湖没有受到明显的汞污染。沉积物中的汞剖面表明,流域的能源需求和政策管理影响了其沉积物中的汞积累。基于菲克第一定律和沉积速率,估算了溶解态 Hg 从沉积物向表层水的扩散通量和积累通量。根据一年的估算,约有 10%-13%的沉积物中的 Hg 可以重新释放到表层水中。从沉积物中扩散出来的 Hg 占表层水中 Hg 的 7.9%-16%。本研究的结果提高了对水体污染来源的认识,使研究人员能够关注沉积物对浅水湖泊水体污染的贡献。

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