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在高纯度LaNiO中观察反铁磁量子临界点

Observation of an antiferromagnetic quantum critical point in high-purity LaNiO.

作者信息

Liu Changjiang, Humbert Vincent F C, Bretz-Sullivan Terence M, Wang Gensheng, Hong Deshun, Wrobel Friederike, Zhang Jianjie, Hoffman Jason D, Pearson John E, Jiang J Samuel, Chang Clarence, Suslov Alexey, Mason Nadya, Norman M R, Bhattacharya Anand

机构信息

Materials Science Division, Argonne National Laboratory, Lemont, IL, 60439, USA.

Department of Physics, University of Illinois at Urbana-Champaign, Urbana, IL, 61801, USA.

出版信息

Nat Commun. 2020 Mar 16;11(1):1402. doi: 10.1038/s41467-020-15143-w.

Abstract

Amongst the rare-earth perovskite nickelates, LaNiO (LNO) is an exception. While the former have insulating and antiferromagnetic ground states, LNO remains metallic and non-magnetic down to the lowest temperatures. It is believed that LNO is a strange metal, on the verge of an antiferromagnetic instability. Our work suggests that LNO is a quantum critical metal, close to an antiferromagnetic quantum critical point (QCP). The QCP behavior in LNO is manifested in epitaxial thin films with unprecedented high purities. We find that the temperature and magnetic field dependences of the resistivity of LNO at low temperatures are consistent with scatterings of charge carriers from weak disorder and quantum fluctuations of an antiferromagnetic nature. Furthermore, we find that the introduction of a small concentration of magnetic impurities qualitatively changes the magnetotransport properties of LNO, resembling that found in some heavy-fermion Kondo lattice systems in the vicinity of an antiferromagnetic QCP.

摘要

在稀土钙钛矿镍酸盐中,氧化镧镍(LNO)是个例外。虽然前者具有绝缘和反铁磁基态,但LNO在极低温度下仍保持金属性且无磁性。人们认为LNO是一种奇异金属,处于反铁磁不稳定性的边缘。我们的研究表明LNO是一种量子临界金属,接近反铁磁量子临界点(QCP)。LNO中的QCP行为在具有前所未有的高纯度的外延薄膜中表现出来。我们发现,LNO在低温下电阻率的温度和磁场依赖性与电荷载流子受弱无序散射以及反铁磁性质的量子涨落一致。此外,我们发现引入少量磁性杂质会定性地改变LNO的磁输运性质,类似于在反铁磁QCP附近的一些重费米子近藤晶格系统中发现的情况。

https://cdn.ncbi.nlm.nih.gov/pmc/blobs/6d8b/7075863/53587322f81d/41467_2020_15143_Fig1_HTML.jpg

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