Department of Nuclear Medicine, Heidelberg University Hospital, Im Neuenheimer Feld 400, 69120, Heidelberg, Germany.
Institute of Pharmacy and Molecular Biotechnology, Heidelberg University, Germany.
Angew Chem Int Ed Engl. 2020 Jun 2;59(23):8823-8827. doi: 10.1002/anie.202002727. Epub 2020 Apr 21.
Multidrug-resistant bacteria represent one of the biggest challenges facing modern medicine. The increasing prevalence of glycopeptide resistance compromises the efficacy of vancomycin, for a long time considered as the last resort for the treatment of resistant bacteria. To reestablish its activity, polycationic peptides were conjugated to vancomycin. By site-specific conjugation, derivatives that bear the peptide moiety at four different sites of the antibiotic were synthesized. The most potent compounds exhibited an approximately 1000-fold increased antimicrobial activity and were able to overcome the most important types of vancomycin resistance. Additional blocking experiments using d-Ala-d-Ala revealed a mode of action beyond inhibition of cell-wall formation. The antimicrobial potential of the lead candidate FU002 for bacterial infection treatments could be demonstrated in an in vivo study. Molecular imaging and biodistribution studies revealed that conjugation engenders superior pharmacokinetics.
耐多药细菌是现代医学面临的最大挑战之一。糖肽类耐药性的日益流行损害了万古霉素的疗效,万古霉素长期以来被认为是治疗耐药菌的最后手段。为了恢复其活性,将聚阳离子肽与万古霉素连接。通过定点连接,合成了在抗生素的四个不同部位带有肽部分的衍生物。最有效的化合物表现出大约 1000 倍的增强抗菌活性,并能够克服最重要类型的万古霉素耐药性。使用 d-Ala-d-Ala 的附加阻断实验揭示了一种作用模式,超出了抑制细胞壁形成的作用模式。先导候选物 FU002 用于细菌感染治疗的抗菌潜力可以在体内研究中得到证明。分子成像和生物分布研究表明,连接产生了更好的药代动力学。