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硼酸盐、碳酸盐和硝酸盐中霰石、方解石和球霰石型结构的红外研究

Infrared Studies of Aragonite, Calcite, and Vaterite Type Structures in the Borates, Carbonates, and Nitrates.

作者信息

Weir C E, Lippincott Ellis R

出版信息

J Res Natl Bur Stand A Phys Chem. 1961 May-Jun;65A(3):173-180. doi: 10.6028/jres.065A.021. Epub 1961 Jun 1.

DOI:10.6028/jres.065A.021
PMID:32196235
原文链接:https://pmc.ncbi.nlm.nih.gov/articles/PMC5287277/
Abstract

Infrared absorption spectra have been obtained on the alkali nitrates, the divalent metal carbonates, and the rare earth borates which assume the aragonite, calcite, or vaterite crystal structures. It was observed that similar structures give rise to analogous spectra except for the carbonate and borates having the vaterite structure. The marked differences observed in these latter spectra are discussed. Frequency shifts produced by cation substitution are ascribed to repulsion between closed electron shells of oxygen atoms. It is concluded that this repulsive force determines the structure type in the rare earth borates.

摘要

已获得具有文石、方解石或球霰石晶体结构的碱金属硝酸盐、二价金属碳酸盐和稀土硼酸盐的红外吸收光谱。观察到，除了具有球霰石结构的碳酸盐和硼酸盐外，相似的结构会产生类似的光谱。讨论了在这些后者的光谱中观察到的明显差异。由阳离子取代产生的频率位移归因于氧原子闭壳层之间的排斥力。得出的结论是，这种排斥力决定了稀土硼酸盐的结构类型。

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https://cdn.ncbi.nlm.nih.gov/pmc/blobs/9625/5287277/563581d8e31d/jresv65an3p173_a1bf12.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/9625/5287277/a1734b925a9d/jresv65an3p173_a1bf13.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/9625/5287277/06bc2c5ef134/jresv65an3p173_a1bf14.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/9625/5287277/368326b6fe90/jresv65an3p173_a1bf15.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/9625/5287277/405b72915fb8/jresv65an3p173_a1bf16.jpg

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