Chen Tingjie, Wu Zhenzeng, Liu Zhiyong, Aladejana John Tosin, Wang Xiaodong Alice, Niu Min, Wei Qihua, Xie Yongqun
College of Materials Science and Engineering, Key Laboratory of Polymer Materials and Products of Universities in Fujian, Fujian University of Technology, Fuzhou, Fujian 350002, P. R. China.
College of Material Engineering, Fujian Agriculture and Forestry University, Fuzhou, Fujian 350002, P. R. China.
ACS Appl Mater Interfaces. 2020 Apr 29;12(17):19511-19518. doi: 10.1021/acsami.0c01815. Epub 2020 Apr 16.
Solar steam generation as a promising solar energy conversion technology has attracted considerable interest in achieving seawater desalination and water purification. Although wood with fast water transportation and excellent heat localization has drawn particular interest in regard to its application for solar steam generation, challenges still remain in terms of its complicated processing techniques and relatively low efficiency. Here, we propose a facile, cost-efficient, and scalable brushing method to prepare an aluminophosphate-treated wood (Wood@AlP) solar steam generation device. The aluminophosphate compound deposited on the wood surface can not only be considered as the Lewis acid catalyst capable of accelerating the formation of the carbon layer but also provide an aluminophosphate layer with a hierarchical porous structure, which is beneficial for broad solar absorption and vapor escape. On the other hand, benefiting from the natural hydrophilicity, low thermal conductivity, and excellent water transportation of wood, the obtained Wood@AlP device can float on seawater and exhibit a high solar thermal efficiency of 90.8% with a net evaporation rate of 1.423 kg m h under 1 sun illumination.
作为一种很有前景的太阳能转换技术,太阳能蒸汽产生在实现海水淡化和水净化方面引起了广泛关注。尽管具有快速输水能力和出色热局域性的木材在太阳能蒸汽产生应用方面备受关注,但其复杂的加工工艺和相对较低的效率仍面临挑战。在此,我们提出一种简便、经济高效且可扩展的涂刷方法来制备磷酸铝处理木材(Wood@AlP)太阳能蒸汽产生装置。沉积在木材表面的磷酸铝化合物不仅可被视为能够加速碳层形成的路易斯酸催化剂,还能提供具有分级多孔结构的磷酸铝层,这有利于广泛的太阳能吸收和蒸汽逸出。另一方面,得益于木材的天然亲水性、低热导率和出色的输水能力,所制备的Wood@AlP装置能够漂浮在海面上,在1个太阳光照强度下展现出90.8%的高太阳能热效率以及1.423 kg m⁻² h⁻¹的净蒸发速率。