Zaitsev A G, Beck A, Jaiswal A K, Singh R, Schneider R, Le Tacon M, Fuchs D
Karlsruhe Institute of Technology, Institute for Solid-State Physics, Karlsruhe, Germany.
Indian Institute of Technology Delhi, Department of Physics, New Delhi 110016, India.
J Phys Condens Matter. 2020 May 22;32(34). doi: 10.1088/1361-648X/ab8a9e.
Iridate oxides display exotic physical properties that arise from the interplay between a large spin-orbit coupling and electron correlations. Here, we present a comprehensive study of the effects of hydrostatic pressure on the electronic transport properties of SrIrO(SIO), a system that has recently attracted a lot of attention as potential correlated Dirac semimetal. Our investigations on untwinned thin films of SIO reveal that the electrical resistivity of this material is intrinsically anisotropic and controlled by the orthorhombic distortion of the perovskite unit cell. These effects provide another evidence for the strong coupling between the electronic and lattice degrees of freedom in this class of compounds. Upon increasing pressure, a systematic increase of the transport anisotropies is observed. The anomalous pressure-induced changes of the resistivity cannot be accounted for by the pressure dependence of the density of the electron charge carriers, as inferred from Hall effect measurements. Moreover, pressure-induced rotations of the IrOoctahedra likely occur within the distorted perovskite unit cell and affect electron mobility of this system.
铱酸盐氧化物展现出源于大自旋轨道耦合与电子关联相互作用的奇特物理性质。在此,我们对静水压力对SrIrO(SIO)电子输运性质的影响进行了全面研究,SIO作为一种潜在的关联狄拉克半金属体系,最近备受关注。我们对SIO非孪晶薄膜的研究表明,这种材料的电阻率本质上是各向异性的,并且由钙钛矿晶胞的正交畸变所控制。这些效应为这类化合物中电子与晶格自由度之间的强耦合提供了另一个证据。随着压力增加,观察到输运各向异性有系统性增加。从霍尔效应测量推断,电阻率的异常压力诱导变化无法用电子电荷载流子密度的压力依赖性来解释。此外,压力诱导的IrO八面体旋转可能发生在畸变的钙钛矿晶胞内,并影响该体系的电子迁移率。