State Key Laboratory of Silicate Materials for Architectures, Wuhan University of Technology, Wuhan 430070, China.
State Key Laboratory of Silicate Materials for Architectures, Wuhan University of Technology, Wuhan 430070, China; Department of Civil and Environmental Engineering, Norwegian University of Science and Technology, 7491 Trondheim, Norway.
J Hazard Mater. 2020 Nov 5;398:122904. doi: 10.1016/j.jhazmat.2020.122904. Epub 2020 May 15.
Volatile organic compounds (VOCs) release from asphalt pavement construction is a potential emission source. The detailed emission behaviors were simulated in the laboratory, and the corresponding environmental impact was investigated as well. A set of dedicated devices were applied to mirror 3 representative scenarios namely mixture plant, transportation and paving processes with VOCs emission concentrations varied from 4.24 mg/m to 104.16 mg/m. Ozone formation potential (OFP) and secondary organic aerosol (SOA) were built to evaluate the environmental impact, indicating that the reactive ability differed in the specified substances. The alkenes (n ≤ 4) and aldehydes, alkanes (n ≥ 6) and alkylbenzenes with relative lower concentration were the main sources for the OFP and SOA generation, and they contributed to more than 62% OFP and 97% SOA respectively. The top 10 contributors to concentration, OFP and SOA had been identified. For the complex species existed in VOCs emission and the lack of VOCs control standards, this study provided possible access to screen priority-controlled pollutants based on information entropy method, in terms of both environmental and human health impact. In addition, the first-class priority-controlled species had been determined, urgently needing more attention in the future VOCs management during asphalt pavement construction.
挥发性有机化合物(VOCs)从沥青路面施工中释放是一个潜在的排放源。本文在实验室中模拟了详细的排放行为,并研究了相应的环境影响。应用了一套专用设备来模拟 3 种具有代表性的场景,即混合料厂、运输和铺设过程,VOCs 排放浓度从 4.24mg/m 到 104.16mg/m 不等。建立了臭氧形成潜力(OFP)和二次有机气溶胶(SOA)来评估环境影响,表明指定物质的反应能力不同。具有较低浓度的烯烃(n ≤ 4)和醛类、烷烃(n ≥ 6)和烷基苯是 OFP 和 SOA 生成的主要来源,它们分别对超过 62%的 OFP 和 97%的 SOA 有贡献。已经确定了对浓度、OFP 和 SOA 贡献最大的前 10 种物质。对于 VOCs 排放中存在的复杂物质和缺乏 VOCs 控制标准,本研究提供了一种基于信息熵法筛选优先控制污染物的可能途径,从环境和人类健康影响两个方面考虑。此外,已经确定了一类优先控制的物质,在未来的沥青路面施工 VOCs 管理中需要更加关注。