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利用正定矩阵因子分解受体模型技术研究中国西北干旱区北川河流域河流水质时空分布及污染源解析

Spatiotemporal Patterns in River Water Quality and Pollution Source Apportionment in the Arid Beichuan River Basin of Northwestern China Using Positive Matrix Factorization Receptor Modeling Techniques.

机构信息

College of Geology and Environment, Xi'an University of Science and Technology, Xi'an 710054, China.

Hebei and China Geological Survey Key Laboratory of Groundwater Remediation, Institute of Hydrogeology and Environmental Geology, Chinese Academy of Geological Sciences, Shijiazhuang 050061, China.

出版信息

Int J Environ Res Public Health. 2020 Jul 13;17(14):5015. doi: 10.3390/ijerph17145015.

Abstract

Deteriorating surface water quality has become an important environmental problem in China. In this study, river water quality was monitored in July (wet season) and October (dry season) 2019 at 26 sites, and a water quality index (WQI) and positive matrix factorization (PMF) model were used to assess surface water quality and identify pollution sources in the Beichuan River basin, Qinghai Province, China. The results showed that 53.85% and 76.92% of TN, 11.54% and 34.62% of TP, 65.38% and 76.92% of Fe, and 11.54% and 15.38% of Mn samples in the dry and wet seasons, respectively, exceeded the Chinese Government's Grade III standards for surface water quality. The spatial variation in water quality showed that it gradually deteriorated from upstream to downstream as a result of human activity. The temporal variation showed that water quality was poorer in the wet season than in the dry season because of the rainfall runoff effect. The PMF model outputs showed that the primary sources of pollution in the wet season were mineral weathering and organic pollution sources, domestic and industrial sewage, and agricultural and urban non-point pollution sources. However, in the dry season, the primary sources were mineral weathering and organic pollution sources, industrial sewage, and domestic sewage. Our results suggest that the point pollution sources (domestic and industrial sewage) should be more strictly controlled, as a priority, in order to prevent the continued deterioration in water quality.

摘要

地表水质恶化已成为中国的一个重要环境问题。本研究于 2019 年 7 月(雨季)和 10 月(旱季)在 26 个站点监测了河水水质,采用水质指数(WQI)和正定矩阵因子分析(PMF)模型评估了青海省北川河流域地表水水质,并识别了污染源。结果表明,TN 的 53.85%和 76.92%、TP 的 11.54%和 34.62%、Fe 的 65.38%和 76.92%以及 Mn 的 11.54%和 15.38%样本在干湿两季均超过了中国地表水环境质量Ⅲ类标准。水质的空间变化表明,由于人类活动的影响,水质从上游到下游逐渐恶化。时间变化表明,由于降雨径流的影响,雨季水质比旱季差。PMF 模型输出表明,雨季的主要污染来源是矿物风化和有机污染源、生活和工业污水以及农业和城市非点源污染。然而,在旱季,主要污染源是矿物风化和有机污染源、工业污水和生活污水。研究结果表明,应更加严格地控制点污染源(生活和工业污水),以防止水质的持续恶化。

https://cdn.ncbi.nlm.nih.gov/pmc/blobs/d525/7399880/f697dc0fa317/ijerph-17-05015-g001.jpg

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