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具有随机重置的扩散的实验实现

Experimental Realization of Diffusion with Stochastic Resetting.

作者信息

Tal-Friedman Ofir, Pal Arnab, Sekhon Amandeep, Reuveni Shlomi, Roichman Yael

机构信息

School of Physics & Astronomy, Raymond and Beverly Sackler Faculty of Exact Sciences, Tel Aviv University, Tel Aviv 6997801, Israel.

School of Chemistry, The Center for Physics and Chemistry of Living Systems, & The Mark Ratner Institute for Single Molecule Chemistry, Tel Aviv University, Tel Aviv 6997801, Israel.

出版信息

J Phys Chem Lett. 2020 Sep 3;11(17):7350-7355. doi: 10.1021/acs.jpclett.0c02122. Epub 2020 Aug 24.

DOI:10.1021/acs.jpclett.0c02122
PMID:32787296
原文链接:https://pmc.ncbi.nlm.nih.gov/articles/PMC7586404/
Abstract

Stochastic resetting is prevalent in natural and man-made systems, giving rise to a long series of nonequilibrium phenomena. Diffusion with stochastic resetting serves as a paradigmatic model to study these phenomena, but the lack of a well-controlled platform by which this process can be studied experimentally has been a major impediment to research in the field. Here, we report the experimental realization of colloidal particle diffusion and resetting via holographic optical tweezers. We provide the first experimental corroboration of central theoretical results and go on to measure the energetic cost of resetting in steady-state and first-passage scenarios. In both cases, we show that this cost cannot be made arbitrarily small because of fundamental constraints on realistic resetting protocols. The methods developed herein open the door to future experimental study of resetting phenomena beyond diffusion.

摘要

随机重置在自然和人造系统中普遍存在,引发了一系列非平衡现象。具有随机重置的扩散是研究这些现象的典型模型,但缺乏一个可以通过实验研究该过程的良好控制平台一直是该领域研究的主要障碍。在此,我们报告了通过全息光镊实现胶体粒子扩散和重置的实验。我们首次对核心理论结果进行了实验验证,并继续测量稳态和首次通过情况下重置的能量成本。在这两种情况下,我们都表明,由于对现实重置协议的基本限制,这种成本不能被任意降低。本文开发的方法为未来超越扩散的重置现象实验研究打开了大门。

https://cdn.ncbi.nlm.nih.gov/pmc/blobs/33bc/7586404/604743f08f55/jz0c02122_0005.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/33bc/7586404/f68be46ac40d/jz0c02122_0001.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/33bc/7586404/ede5fc5ee2e6/jz0c02122_0002.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/33bc/7586404/f57cb3f3cc80/jz0c02122_0003.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/33bc/7586404/c5544a2da31f/jz0c02122_0004.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/33bc/7586404/604743f08f55/jz0c02122_0005.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/33bc/7586404/f68be46ac40d/jz0c02122_0001.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/33bc/7586404/ede5fc5ee2e6/jz0c02122_0002.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/33bc/7586404/f57cb3f3cc80/jz0c02122_0003.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/33bc/7586404/c5544a2da31f/jz0c02122_0004.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/33bc/7586404/604743f08f55/jz0c02122_0005.jpg

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本文引用的文献

1
Resetting processes with noninstantaneous return.具有非瞬时返回的重置过程。
Phys Rev E. 2020 May;101(5-1):052130. doi: 10.1103/PhysRevE.101.052130.
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Work Fluctuations and Jarzynski Equality in Stochastic Resetting.随机重置中的工作涨落和雅可比等式。
Phys Rev Lett. 2020 Mar 20;124(11):110608. doi: 10.1103/PhysRevLett.124.110608.
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Time-dependent density of diffusion with stochastic resetting is invariant to return speed.具有随机重置的扩散的时变密度与返回速度无关。
Proc Natl Acad Sci U S A. 2025 Jan 7;122(1):e2402912121. doi: 10.1073/pnas.2402912121. Epub 2025 Jan 2.
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Fractional Telegrapher's Equation under Resetting: Non-Equilibrium Stationary States and First-Passage Times.重置条件下的分数阶电报方程:非平衡稳态与首次通过时间
Entropy (Basel). 2024 Aug 5;26(8):665. doi: 10.3390/e26080665.
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Random Walks on Comb-like Structures under Stochastic Resetting.随机重置下梳状结构上的随机游走
Entropy (Basel). 2023 Nov 9;25(11):1529. doi: 10.3390/e25111529.
6
Mitigating long queues and waiting times with service resetting.通过服务重置来缓解长队和等待时间。
PNAS Nexus. 2022 Jul 1;1(3):pgac070. doi: 10.1093/pnasnexus/pgac070. eCollection 2022 Jul.
7
Stochastic Resetting for Enhanced Sampling.随机重置增强采样。
J Phys Chem Lett. 2022 Dec 8;13(48):11230-11236. doi: 10.1021/acs.jpclett.2c03055. Epub 2022 Nov 29.
Phys Rev E. 2019 Oct;100(4-1):040101. doi: 10.1103/PhysRevE.100.040101.
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Transport properties of random walks under stochastic noninstantaneous resetting.随机非瞬时重置下随机游走的输运性质。
Phys Rev E. 2019 Oct;100(4-1):042104. doi: 10.1103/PhysRevE.100.042104.
5
Symmetric exclusion process under stochastic resetting.随机重置下的对称排斥过程。
Phys Rev E. 2019 Sep;100(3-1):032136. doi: 10.1103/PhysRevE.100.032136.
6
Nonrenewal resetting of scaled Brownian motion.规模布朗运动的非更新重置。
Phys Rev E. 2019 Jul;100(1-1):012119. doi: 10.1103/PhysRevE.100.012119.
7
Scaled Brownian motion with renewal resetting.带重置更新的标度布朗运动。
Phys Rev E. 2019 Jul;100(1-1):012120. doi: 10.1103/PhysRevE.100.012120.
8
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Dev Cell. 2019 Jun 17;49(6):894-906.e12. doi: 10.1016/j.devcel.2019.04.031. Epub 2019 May 16.
9
First passage under stochastic resetting in an interval.区间内随机重置下的首次通过
Phys Rev E. 2019 Mar;99(3-1):032123. doi: 10.1103/PhysRevE.99.032123.
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First Passage under Restart with Branching.分支重启动下的首次穿越。
Phys Rev Lett. 2019 Jan 18;122(2):020602. doi: 10.1103/PhysRevLett.122.020602.