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俄罗斯秋明市城市街道灰尘中潜在有毒元素和多环芳烃的污染状况及对人类健康的风险评估。

Pollution status and human health risk assessment of potentially toxic elements and polycyclic aromatic hydrocarbons in urban street dust of Tyumen city, Russia.

机构信息

Southern Federal University, Rostov-on-Don, Russian Federation.

University of Tyumen, 6 Volodarskogo St., Tyumen, Russian Federation.

出版信息

Environ Geochem Health. 2022 Feb;44(2):409-432. doi: 10.1007/s10653-020-00692-2. Epub 2020 Aug 14.

Abstract

This study investigated levels and sources of pollution and potential health risks associated with potentially toxic elements (PTEs) and polycyclic aromatic hydrocarbons (PAHs) in urban street dust collected from Tyumen city, a large transport centre with one of the highest motorization rates in Russia. Twenty street dust samples were collected from four grades of roads in five different land use areas. Research methods included measurements of physical and chemical properties of street dust, concentrations of 18 PTEs using inductively coupled plasma mass spectrometry, 12 PAHs using high-performance liquid chromatography, and statistical analysis of the data. Concentrations of Ni, Cr, Sb, and Mo, as well as medium and high molecular weight PAHs in urban street dust, were notably higher than in soils within the city, which indicates that transport is the main source of these elements. Concentrations of Cu, Cd, Pb, Zn, Mn, and As in street dust of Tyumen were lower compared to many large cities, while Cr, Ni, and Co were higher. Concentrations of PAH were comparable to other large nonindustrial cities. Total contamination of street dust by both PTEs and PAHs showed more robust relationships with the number of roadway lanes rather than land use. The estimated carcinogenic risks were low in 70% of samples and medium in 30% of samples. Noncarcinogenic risks were attributed to exposure to Co, Ni, V, and As. The total noncarcinogenic risk for adults was found to be negligible, while the risk was found to be moderate for children.

摘要

本研究调查了从俄罗斯机动车保有率最高的城市之一秋明市收集的城市街道灰尘中与潜在有毒元素(PTE)和多环芳烃(PAH)相关的污染水平和来源,以及潜在健康风险。从五个不同土地利用区域的四条道路等级采集了 20 个街道灰尘样本。研究方法包括街道灰尘物理化学性质的测量、电感耦合等离子体质谱法测定 18 种 PTE 的浓度、高效液相色谱法测定 12 种 PAH 的浓度,以及数据的统计分析。城市街道灰尘中的 Ni、Cr、Sb 和 Mo 以及中高分子量 PAH 的浓度明显高于城市内土壤,这表明交通是这些元素的主要来源。与许多大城市相比,秋明市街道灰尘中的 Cu、Cd、Pb、Zn、Mn 和 As 浓度较低,而 Cr、Ni 和 Co 浓度较高。PAH 的浓度与其他大型非工业城市相当。PTE 和 PAH 对街道灰尘的总污染与道路车道数量的关系比土地利用更为密切。在 70%的样本中,估计的致癌风险较低,在 30%的样本中为中等。非致癌风险归因于 Co、Ni、V 和 As 的暴露。成年人的总非致癌风险被认为可以忽略不计,而儿童的风险被认为是中等的。

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