Department of Earth Sciences, College of Sciences, Shiraz University, Shiraz, Iran.
Environ Geochem Health. 2021 Jan;43(1):485-519. doi: 10.1007/s10653-020-00682-4. Epub 2020 Oct 9.
Contamination level, source, and ecological-health risk of potentially toxic elements (PTEs) and polycyclic aromatic hydrocarbons (PAHs) in the street dust of Yazd, a central capital city in Iran, were investigated for the first time regarding samples collected from 21 sites. Geochemical indices pointed out an enrichment trend of [Formula: see text] and an ecological risk trend of [Formula: see text]. The ecological risk indices of PAHs reflected high ecological risk for pyrene (Pyr). The statistical approach along with the isomeric ratios of PAHs suggested that the traffic-related sources, such as wearing of tires and brake pads, and the vehicular exhaust emissions were greatly responsible for the elevated concentrations of Pb, Cu, Sb, and PAHs, while Al, Ni, Co, V, Mn, As, and, to a lesser extent, Fe, Zn, Mo, and Cr were mainly influenced by geogenic sources. The human health risk assessment of PTEs and PAHs reflected that As, Cr, and Pb pose the highest non-carcinogenic risk in adults and children, compared with other PTEs and also PAHs. The carcinogenic health risk of Pb in the children and PAHs in both subpopulations was high for cancer development.
首次针对伊朗中部首都亚兹德市的 21 个地点采集的街道灰尘样本,研究了潜在有毒元素 (PTE) 和多环芳烃 (PAH) 的污染水平、来源和生态健康风险。地球化学指标指出 [Formula: see text] 的富集趋势和 [Formula: see text] 的生态风险趋势。PAHs 的生态风险指数反映了苝 (Pyr) 的高生态风险。统计方法以及 PAHs 的同系物比值表明,与交通相关的来源,如轮胎和刹车片的磨损以及车辆排放的废气,对 Pb、Cu、Sb 和 PAHs 的高浓度负有重大责任,而 Al、Ni、Co、V、Mn、As 以及在较小程度上 Fe、Zn、Mo 和 Cr 主要受到地球成因来源的影响。PTE 和 PAHs 的人体健康风险评估表明,与其他 PTE 相比,As、Cr 和 Pb 对成人和儿童造成的非致癌风险最高。儿童体内的 Pb 和两个亚群体内的 PAHs 的致癌健康风险对癌症的发展都很高。