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开发新型反硝化亚硝积累除磷(DNAPR)工艺,作为一种替代预处理方法,以实现主流厌氧氨氧化。

Development of novel denitrifying nitrite accumulation and phosphorus removal (DNAPR) process for offering an alternative pretreatment to achieve mainstream Anammox.

机构信息

School of Environmental Science and Engineering, Qingdao University, Qingdao 266071, PR China.

School of Environmental Science and Engineering, Qingdao University, Qingdao 266071, PR China.

出版信息

Bioresour Technol. 2021 Jan;319:124164. doi: 10.1016/j.biortech.2020.124164. Epub 2020 Sep 24.

DOI:10.1016/j.biortech.2020.124164
PMID:33002785
Abstract

For achieving mainstream anaerobic ammonium oxidation (Anammox), there is a need to achieve organic carbon and phosphorus removal meanwhile supplying nitrite (NO-N). Based on this demand, a novel anaerobic/anoxic/aerobic operated denitrifying nitrite accumulation and phosphorus removal (DNAPR) process was proposed for treating synthetic municipal and nitrate (NO-N) wastewaters simultaneously (volume ratio of 5:1). By adjusting influent composition, discharging anaerobic-end supernatant, shortening anoxic duration, and adding a short aerobic stage, DNAPR process achieved promising and stable nitrate-to-nitrite transformation (78.35%) and phosphorus removal (98.34%) performance. Moreover, effluent with chemical oxygen demand of 16.63 mg/L, nitrite of 54.16 mg/L, orthophosphate of 0.37 mg/L, and nitrite to ammonia ratio of 1.3 were finally obtained after 141-day operation. Microbiological analysis showed that Thauera (34.9%) and unclassified_f_Rhodobacteraceae (6.79%) were both responsible for DNAPR. Therefore, DNAPR, serving as promising alternative pretreatment, might possess significance for achieving mainstream Anammox.

摘要

为实现主流厌氧氨氧化(Anammox),需要同时去除有机碳和磷,并供应亚硝酸盐(NO-N)。基于这一需求,提出了一种新型的厌氧/缺氧/好氧脱氮亚硝酸盐积累和除磷(DNAPR)工艺,用于同时处理合成城市和硝酸盐(NO-N)废水(体积比为 5:1)。通过调整进水成分、排放厌氧末端上清液、缩短缺氧时间和添加短好氧阶段,DNAPR 工艺实现了有希望且稳定的硝酸盐到亚硝酸盐的转化(78.35%)和磷去除(98.34%)性能。此外,经过 141 天的运行,最终出水的化学需氧量为 16.63mg/L、亚硝酸盐为 54.16mg/L、正磷酸盐为 0.37mg/L、亚硝酸盐与氨的比例为 1.3。微生物分析表明,Thauera(34.9%)和未分类_f_Rhodobacteraceae(6.79%)都负责 DNAPR。因此,DNAPR 作为一种有前途的替代预处理方法,可能对实现主流 Anammox 具有重要意义。

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