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掀起波澜:提高常规污水处理厂对内分泌干扰化合物(EDCs)的去除性能:它们的共轭物很重要。

Making waves: Improving removal performance of conventional wastewater treatment plants on endocrine disrupting compounds (EDCs): their conjugates matter.

机构信息

School of Environment and Energy, South China University of Technology, Guangzhou, 510006, Guangdong, China; Key Lab Pollution Control & Ecosystem Restoration in Industry Cluster, Ministry of Education, Guangzhou 510006, Guangdong, China; Guangdong Provincial Key Laboratory of Solid Wastes Pollution Control and Recycling, Guangzhou, 510006, Guangdong, China; Guangdong Provincial Engineering and Technology Research Center for Environment Risk Prevention and Emergency Disposal, South China University of Technology, Guangzhou, 510006, Guangdong, China.

Key Lab Pollution Control & Ecosystem Restoration in Industry Cluster, Ministry of Education, Guangzhou 510006, Guangdong, China.

出版信息

Water Res. 2021 Jan 1;188:116469. doi: 10.1016/j.watres.2020.116469. Epub 2020 Sep 28.

Abstract

Endocrine disrupting compounds (EDCs) are well known emerging contaminants, which have the capacity to elicit negative effects on endocrine systems of both humans and wildlife. As the conventional wastewater treatment plants cannot stably remove these EDCs, post-treatment with advanced chemical oxidation methods such as ozonation are proven effective to further remove EDCs, but this additional treatment increase the wastewater treatment cost, which is impractical for worldwide application. To find potential alternative effective method, this work presents the importance of EDCs conjugates. Specifically, two important facts are described: 1) concentrations of EDCs conjugates in raw municipal wastewater vary with temperature, and their existence results in underestimated removal performance of WWTPs; 2) Strategies to enhance the cleavage rates of EDCs conjugates are most effective to improve the observed removal performance of conventional WWTPs on EDCs. Further work should be performed to check whether effective solutions can be found to increase their cleavage rates.

摘要

内分泌干扰化合物 (EDCs) 是众所周知的新兴污染物,它们有能力对人类和野生动物的内分泌系统产生负面影响。由于传统的废水处理厂不能稳定地去除这些 EDCs,因此臭氧等高级化学氧化方法的后处理被证明可以有效地进一步去除 EDCs,但这种额外的处理会增加废水处理成本,在全球范围内应用是不切实际的。为了寻找潜在的替代有效方法,本工作介绍了 EDCs 缀合物的重要性。具体来说,描述了两个重要事实:1)原始城市废水中 EDCs 缀合物的浓度随温度变化,其存在导致 WWTPs 的去除性能被低估;2)增强 EDCs 缀合物的裂解速率的策略对提高传统 WWTPs 对 EDCs 的观察去除性能最有效。应进一步开展工作,以检查是否可以找到有效解决方案来提高它们的裂解速率。

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