Sun Jia-Ning, Xie Shao-Dong
College of Environmental Sciences and Engineering, Peking University, Beijing 100871, China.
Huan Jing Ke Xue. 2020 Nov 8;41(11):4874-4884. doi: 10.13227/j.hjkx.202002002.
To accurately identify and locate ambient volatile organic compounds(VOCs)emission sources in industrial parks, a continuous online GC-FID method was used to monitor 43 kinds of VOCs on an hourly basis during January 2017 at five sites in an industrial park. A statistical analysis and a PMF model were used to analyze the sources of VOCs, and by combining with CPF and enterprise emission information, the location of each pollution source was accurately identified. The average VOCs concentration was 56.40×10 and the highest concentration of alkanes was observed at four sites, with the exception of one site. Ethane, propane, ethylene, toluene, isobutane, n-butane, and acetylene were the main contributors. Ambient VOCs in the park mainly derives from five sources:urban transmission, butane leakage, process emissions, storage tank emissions, and ethylene synthesis. The enterprises in the zone B1, A1-A3, C1-C2, F4, E4-E6, F4-F6, and the canal loading and unloading area are the main emission areas of the pollution sources. Using online monitoring data, the research combined a PMF model, meteorological conditions, and corporate emissions information to achieve precise positioning of the pollution sources of VOCs in the industrial park, thus providing a basis for the supervision and management of corporate emissions in industrial parks.
为准确识别和定位工业园区内环境挥发性有机化合物(VOCs)排放源,采用连续在线气相色谱 - 火焰离子化检测法(GC - FID)于2017年1月对某工业园区内5个点位的43种VOCs进行 hourly 监测。运用统计分析和正定矩阵因子分解(PMF)模型分析VOCs来源,并结合浓度 - 路径指纹(CPF)和企业排放信息,精准识别各污染源位置。VOCs平均浓度为56.40×10(此处原文似乎有误,单位不完整),除一个点位外,其他四个点位烷烃浓度最高。乙烷、丙烷、乙烯、甲苯、异丁烷、正丁烷和乙炔为主要贡献物种。园区内环境VOCs主要来源于城市传输、丁烷泄漏、工艺排放、储罐排放和乙烯合成。B1区、A1 - A3区、C1 - C2区、F4区、E4 - E6区、F4 - F6区以及运河装卸区的企业是污染源的主要排放区域。该研究利用在线监测数据,结合PMF模型、气象条件和企业排放信息,实现了工业园区内VOCs污染源的精准定位,从而为工业园区企业排放监管提供依据。 (注:原文中“hourly”疑为“每小时地”之意,但结合语境此处翻译较难完全准确通顺,整体译文尽量忠实原文并调整了部分表述使其更符合中文表达习惯)