Du Ying-Ying, Chen Jun, Zhang Jia-Luo, Gan Gui-Cheng, Liu Yu-Cun, Su Ming-Xu, Lou Sheng-Rong, Zhou Min, Tao Shi-Kang, Qiao Li-Ping
Shanghai Key Laboratory of Multiphase Flow and Heat Transfer in Power Engineering, School of Energy and Power Engineering, University of Shanghai for Science and Technology, Shanghai 200093, China.
State Environmental Protection Key Laboratory of Formation and Prevention of Urban Air Pollution Complex, Shanghai Academy of Environmental Sciences, Shanghai 200233, China.
Huan Jing Ke Xue. 2020 Sep 8;41(9):3932-3940. doi: 10.13227/j.hjkx.201911271.
In a recent field campaign focused on air quality study, aerosol optical properties, particle number concentration, and PM components were monitored in Changzhou, Jiangsu Province, from May 27 to June 27, 2019. An array of instruments were deployed that included scanning mobility particle size spectrometer (SMPS), aethalometer (AE33), cavity attenuation phase shift single albedo monitor (CAPS-ALB), monitor for aerosols and gases in ambient air (MARGA) and RT-4 organic carbon/elemental carbon (OC/EC) carbon analyzer to study the ① changes in chemical composition and optical parameters of the new particles generated during the campaign period. ② comparison of the aerosol extinction coefficient recorded by these instruments and measured value in the reconstruction of IMPROVE (interagency monitoring of protected visual environment) and the calculated coefficient using MIE theory model were carried out. During the entire campaign, two new particle generation events were observed and also found that the particle size continued to increase from 4 nm to 64 nm. It was monitored that in the initial stage of new particle generation, sulfate contributed greatly. The measured average aerosol extinction coefficient during the period of particle generation, using these instruments was 95.40 Mm, while the average aerosol extinction reconstruction using the IMPROVE model was observed to be 140.20 Mm. The theoretical calculations based on Mie theory model yielded an average extinction coefficient of 93.54 Mm. It was found that the average aerosol extinction in Changzhou is lower than the average value of the urban aerosol extinction coefficient, which is measured to be 300 Mm in China, during this period. The deployment of multiple instruments in a single campaign is more desirable because the combination of all observations helped in better characterization of the physicochemical properties of ambient aerosols from various aspects, including particle size spectrum and chemical composition.
