School of Environmental and Municipal Engineering, Lanzhou Jiaotong University, Lanzhou, People's Republic of China.
Key Laboratory of Yellow River Water Environment in Gansu Province, Lanzhou, People's Republic of China.
J Air Waste Manag Assoc. 2021 Mar;71(3):392-399. doi: 10.1080/10962247.2020.1843563. Epub 2021 Jan 25.
The mobility and bioavailability of heavy metals in sewage sludge are the major risks to utilize for agricultural application. In this study, the chemical speciation of Cu, Ni, Cr, and Zn in the Lanzhou municipal sewage sludge were investigated with the addition of a natural attapulgite. The influences of attapulgite amendment in sewage sludge on heavy metals stabilization were evaluated by investigating the leaching procedure and sequential chemical extraction experiments. The sequential extraction procedure described by European Community Bureau of Reference was used in sludge to determine the distribution of heavy metal species. The addition of attapulgite accelerated more reducible speciation of all metals transformed into residual speciation evidently. It reduced the leaching content of metals significantly and decreased the ecotoxicity accounted for the germination index values climbed rapidly with increased attapulgite addition.: This research developed a method to stabilize heavy metals in municipal sewage sludge with clay. The activated attapulgite improved the treatment of sewage sludge containing heavy metals, and reduced the environmental risk of heavy metals.
城市污泥中重金属的迁移性和生物可利用性是其农用的主要风险因素。本研究采用天然凹凸棒石对兰州市城市污泥中 Cu、Ni、Cr 和 Zn 的化学形态进行了研究。通过浸出程序和顺序化学提取实验,评估了凹凸棒石改良污泥对重金属稳定化的影响。采用欧洲共同体局参考方法对污泥中的重金属形态进行了测定。添加凹凸棒石后,所有金属的可还原形态明显加速转化为稳定的残余形态。这显著降低了金属的浸出含量,降低了生态毒性,因为发芽指数值随着凹凸棒石添加量的增加而迅速上升。本研究开发了一种用粘土稳定城市污水污泥中重金属的方法。活性凹凸棒石改善了含重金属污泥的处理,降低了重金属的环境风险。