Vaghasiya Jayraj V, Mayorga-Martinez Carmen C, Sofer Zdenek, Pumera Martin
Center for Advanced Functional Nanorobots, Department of Inorganic Chemistry, Faculty of Chemical Technology, University of Chemistry and Technology Prague, Technická 5, Prague 166 28, Czech Republic.
Department of Chemical and Biomolecular Engineering, Yonsei University, 50 Yonseiro, Seodaemun-gu, Seoul 03722, Korea.
ACS Appl Mater Interfaces. 2020 Nov 25;12(47):53039-53048. doi: 10.1021/acsami.0c12879. Epub 2020 Nov 11.
Owing to the rise of miniaturized wearable electronic devices in the last decade, significant demands have arisen to obtain high-performance flexible supercapacitors (FSCs). Recently, a lot of research has been focused on developing smart components of FSCs and integrating them into new device configurations. In this work, FSCs based on a TiC nanosheet (NS) and an organic ionic conductor (OIC)-induced hydrogel as the electrode and the electrolyte, respectively, were used. The FSCs fabricated have three different configurations (sandwich, twisted fiber, and interdigitated) and a comparative study of their electrochemical performance was investigated in terms of cycle stability, bending stability, power density, and energy density. Finally, the experimental validation of practical application was conducted, which suggested excellent electrochemical stability of TiC NS FSCs for driven commercial electronic gadgets. This study presents mechanically robust, lightweight, high-performance FSCs, which can be assembled in different configurations for powering wearable electronic devices.
由于过去十年中微型可穿戴电子设备的兴起,对高性能柔性超级电容器(FSC)的需求大幅增加。最近,许多研究都集中在开发FSC的智能组件并将其集成到新的设备配置中。在这项工作中,分别使用基于TiC纳米片(NS)和有机离子导体(OIC)诱导水凝胶作为电极和电解质的FSC。所制备的FSC具有三种不同的配置(三明治、扭曲纤维和叉指式),并从循环稳定性、弯曲稳定性、功率密度和能量密度方面对其电化学性能进行了对比研究。最后,进行了实际应用的实验验证,结果表明TiC NS FSC在驱动商用电子设备方面具有出色的电化学稳定性。本研究展示了机械坚固、重量轻、高性能的FSC,其可以组装成不同配置以为可穿戴电子设备供电。