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基于金属纳米颗粒修饰的AlGaN多量子阱的安德森局域化实现光谱稳定的深紫外激光器

Anderson Localization Enabled Spectrally Stable Deep-Ultraviolet Laser Based on Metallic Nanoparticle Decorated AlGaN Multiple Quantum Wells.

作者信息

Wu Meng-Jer, Wu Shang-Cheng, Shen Tien-Lin, Liao Yu-Ming, Chen Yang-Fang

机构信息

Department of Physics, National Taiwan University, Taipei 10617, Taiwan.

出版信息

ACS Nano. 2021 Jan 26;15(1):330-337. doi: 10.1021/acsnano.0c04512. Epub 2020 Dec 7.

Abstract

Random lasers exhibit many exotic properties, including chaotic behavior, light localization, broad angular emission, and cost-effective fabrication, which enable them to attract both scientific and industrial interests. However, before the realization of their potential applications, several challenges still remain including the underlying mechanism and controllability due to their inherent multidirectional and chaotic fluctuations. Through more than two decades of collaborative efforts, the discovery of Anderson localization in random lasers provides a plausible route to resolve the difficulties, which enables one to tailor the number of lasing modes and stabilize the emission spectra. However, the related studies are rather rare and only restricted to limited wavelengths. In this study, based on enhanced Anderson localization assisted by surface plasmon resonance, spectrally stable deep-ultraviolet lasing action in AlGaN multiple quantum wells (MQWs) is demonstrated. Our work serves as firm evidence to demonstrate the underlying mechanism of stabilized deep-ultraviolet random laser action that multiple scattering of a light beam in a disordered medium can induce Anderson localization similar to electron behavior. This feature covers the whole spectral range, and it is a universal phenomenon of an electromagnetic wave. Notably, stabilized deep-ultraviolet random laser action has not been demonstrated in all previous studies, even though it has great academic interest and potential application in many areas from environmental protection to biomedical engineering.

摘要

随机激光器具有许多奇异特性,包括混沌行为、光局域化、宽角度发射以及经济高效的制造工艺,这些特性使其在科学界和工业界都备受关注。然而,在其潜在应用得以实现之前,仍存在一些挑战,包括由于其固有的多向性和混沌波动所导致的潜在机制和可控性问题。经过二十多年的共同努力,随机激光器中安德森局域化的发现为解决这些难题提供了一条可行途径,这使得人们能够调整激光模式的数量并稳定发射光谱。然而,相关研究相当稀少,并且仅局限于有限的波长范围。在本研究中,基于表面等离子体共振辅助增强的安德森局域化,实现了AlGaN多量子阱(MQW)中光谱稳定的深紫外激光发射。我们的工作有力地证明了稳定深紫外随机激光发射的潜在机制,即光束在无序介质中的多次散射可诱导类似于电子行为的安德森局域化。这一特性涵盖了整个光谱范围,是电磁波的一种普遍现象。值得注意的是,尽管稳定深紫外随机激光发射在从环境保护到生物医学工程等许多领域具有重大的学术意义和潜在应用价值,但在以往所有研究中均未得到证实。

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