Shneidman Vitaly A
Department of Physics, New Jersey Institute of Technology, Newark, NJ 07102, USA.
Entropy (Basel). 2020 Aug 26;22(9):934. doi: 10.3390/e22090934.
It is shown that in the growth region (above the critical nucleation size) the transient distributions obtained numerically from the Becker-Döring equation (BDE) by Abyzov et al., , , 558, are in accurate correspondence with the matched asymptotic (singular perturbation) solution by Shneidman, , , 1338. The solution is unmodified by "self-consistency" corrections which affect only the steady state rate. Sensitivity of the results to selection of a specific form of the BDE (the "nucleation model") also is briefly discussed.
结果表明,在生长区域(临界成核尺寸以上),阿比佐夫等人从贝克尔 - 多林方程(BDE)数值得到的瞬态分布与施奈德曼的匹配渐近(奇异摄动)解精确对应。该解不受仅影响稳态速率的“自洽性”修正的影响。还简要讨论了结果对BDE特定形式(“成核模型”)选择的敏感性。