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多模有机极化激元激光

Multimode Organic Polariton Lasing.

作者信息

Arnardottir Kristin B, Moilanen Antti J, Strashko Artem, Törmä Päivi, Keeling Jonathan

机构信息

SUPA, School of Physics and Astronomy, University of St Andrews, St Andrews KY16 9SS, United Kingdom.

Department of Applied Physics, Aalto University School of Science, P.O. Box 15100, Aalto FI-00076, Finland.

出版信息

Phys Rev Lett. 2020 Dec 4;125(23):233603. doi: 10.1103/PhysRevLett.125.233603.

Abstract

We present a beyond-mean-field approach to predict the nature of organic polariton lasing, accounting for all relevant photon modes in a planar microcavity. Starting from a microscopic picture, we show how lasing can switch between polaritonic states resonant with the maximal gain, and those at the bottom of the polariton dispersion. We show how the population of nonlasing modes can be found, and by using two-time correlations, we show how the photoluminescence spectrum (of both lasing and nonlasing modes) evolves with pumping and coupling strength, confirming recent experimental work on the origin of blueshift for polariton lasing.

摘要

我们提出了一种超越平均场的方法来预测有机极化激元激光的性质,该方法考虑了平面微腔中所有相关的光子模式。从微观角度出发,我们展示了激光如何在与最大增益共振的极化激元态和极化激元色散底部的态之间切换。我们展示了如何找到非激光模式的布居数,并且通过使用二阶关联,我们展示了(激光和非激光模式的)光致发光光谱如何随泵浦和耦合强度演化,证实了最近关于极化激元激光蓝移起源的实验工作。

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