Maitra Ananyo, Lenz Martin, Voituriez Raphael
Sorbonne Université and CNRS, Laboratoire Jean Perrin, F-75005, Paris, France.
LPTMS, CNRS, Université Paris-Sud, Université Paris-Saclay, 91405 Orsay, France.
Phys Rev Lett. 2020 Dec 4;125(23):238005. doi: 10.1103/PhysRevLett.125.238005.
Active materials, composed of internally driven particles, have properties that are qualitatively distinct from matter at thermal equilibrium. However, the most spectacular departures from equilibrium phase behavior are thought to be confined to systems with polar or nematic asymmetry. In this Letter, we show that such departures are also displayed by more symmetric phases such as hexatics if, in addition, the constituent particles have chiral asymmetry. We show that chiral active hexatics whose rotation rate does not depend on density have giant number fluctuations. If the rotation rate depends on density, the giant number fluctuations are suppressed due to a novel orientation-density sound mode with a linear dispersion which propagates even in the overdamped limit. However, we demonstrate that beyond a finite but large length scale, a chirality and activity-induced relevant nonlinearity invalidates the predictions of the linear theory and destroys the hexatic order. In addition, we show that activity modifies the interactions between defects in the active chiral hexatic phase, making them nonmutual. Finally, to demonstrate the generality of a chiral active hexatic phase we show that it results from the melting of chiral active crystals in finite systems.
由内部驱动粒子组成的活性材料具有与处于热平衡状态的物质在性质上截然不同的特性。然而,人们认为与平衡相行为最显著的偏离仅限于具有极性或向列不对称性的系统。在本信函中,我们表明,如果组成粒子此外还具有手性不对称性,那么这种偏离也会出现在诸如六重态等更对称的相中。我们表明,旋转速率不依赖于密度的手性活性六重态具有巨大的数量涨落。如果旋转速率依赖于密度,由于一种具有线性色散的新型取向 - 密度声模,即使在过阻尼极限下也能传播,巨大的数量涨落就会受到抑制。然而,我们证明,在超过一个有限但很大的长度尺度时,一种手性和活性诱导的相关非线性会使线性理论的预测失效并破坏六重态序。此外,我们表明活性会改变活性手性六重态相中缺陷之间的相互作用,使其不再相互作用。最后,为了证明手性活性六重态相的普遍性,我们表明它是有限系统中手性活性晶体熔化的结果。