Liu Na, Gallaro Cosmo M, Shayan Kamran, Mukherjee Arunabh, Kim Bumho, Hone James, Vamivakas Nick, Strauf Stefan
Department of Physics, Stevens Institute of Technology, Hoboken, New Jersey 07030, USA.
The Institute of Optics, University of Rochester, Rochester, New York 14627, USA and Center for Coherence and Quantum Optics, University of Rochester, Rochester, New York 14627, USA.
Nanoscale. 2021 Jan 21;13(2):832-841. doi: 10.1039/d0nr06632j.
van der Waals ferromagnets have gained significant interest due to their unique ability to provide magnetic response even at the level of a few monolayers. Particularly in combination with 2D semiconductors, such as the transition metal dichalcogenide WSe2, one can create heterostructures that feature unique magneto-optical response in the exciton emission through the magnetic proximity effect. Here we use 0D quantum emitters in WSe2 to probe for the ferromagnetic response in heterostructures with Fe3GT and Fe5GT ferromagnets through an all-optical read-out technique that does not require electrodes. The spectrally narrow spin-doublet of the WSe2 quantum emitters allowed to fully resolve the hysteretic magneto-response in the exciton emission, revealing the characteristic signature of both ferro- and antiferromagnetic proximity coupling that originates from the interplay among Fe3GT or Fe5GT, a thin surface oxide, and the spin doublets of the quantum emitters. Our work highlights the utility of 0D quantum emitters for probing interface magnetic dipoles in vdW heterostructures with high precision. The observed hysteretic magneto response in the exciton emission of quantum emitters adds further new degrees of freedom for spin and g-factor manipulation of quantum states.
范德华铁磁体因其即使在几层单分子层水平也能提供磁响应的独特能力而备受关注。特别是与二维半导体(如过渡金属二硫属化物WSe2)结合时,可以创建通过磁近邻效应在激子发射中具有独特磁光响应的异质结构。在这里,我们利用WSe2中的零维量子发射器,通过一种不需要电极的全光读出技术,探测与Fe3GT和Fe5GT铁磁体构成的异质结构中的铁磁响应。WSe2量子发射器的光谱窄自旋二重态能够完全分辨激子发射中的磁滞磁响应,揭示了源自Fe3GT或Fe5GT、薄表面氧化物以及量子发射器自旋二重态之间相互作用的铁磁和反铁磁近邻耦合的特征信号。我们的工作突出了零维量子发射器在高精度探测范德华异质结构中界面磁偶极子方面的实用性。在量子发射器的激子发射中观察到的磁滞磁响应为量子态的自旋和g因子操纵增加了新的自由度。