Terahertz Spectroscopy of Gas Absorption Using the Superconducting Flux-Flow Oscillator as an Active Source and the Superconducting Integrated Receiver.

We report on the first implementation of a terahertz (THz) source based on a Josephson flux-flow oscillator (FFO) that radiates to open space. The excellent performance of this source and its maturity for practical applications has been demonstrated by the spectroscopy of gas absorption. To study the radiated power, we used a bolometric detection method and additionally calibrated the power by means of pumping the superconductor-insulator-superconductor (SIS) junction, integrated on a single chip with the FFO. For calibration, we developed a program using the SIS-detected power calculations in accordance with the Tien and Gordon model. The power emitted to open space is estimated to be from fractions of µW to several µW in the wide region from 0.25 THz up to 0.75 THz for different designs, with a maximum power of 3.3 µW at 0.34 THz. Next, we used a gas cell and a heterodyne superconducting integrated receiver to trace the absorption lines of water and ammonia with a spectral resolution better than 100 kHz. Our experiment for gas absorption is the first demonstration of the applicability of the FFO as an external active source for different tasks, such as THz spectroscopy, near-field THz imaging and microscopy.