Reactor and Nuclear Systems Division, Oak Ridge National Laboratory, Oak Ridge, TN, 37830, United States.
Idaho National Laboratory, Idaho Falls, ID, 83401, United States.
Appl Radiat Isot. 2021 Mar;169:109494. doi: 10.1016/j.apradiso.2020.109494. Epub 2020 Dec 11.
Domestic production of high specific activity Co was halted after a target rupture in 2012 at the Advanced Test Reactor (ATR). The Isotope Program (IP) within the US Department of Energy (DOE) Office of Science tasked a multilaboratory team of researchers and managers from Oak Ridge and Idaho National Laboratories with the redesign the radioisotope capsule. The objective of this effort was to create a more robust and reliable design, compared to the pre-2012 target. The team successfully completed this task to produce the DOE-IP cobalt (Co) production capsule design. Furthermore, 66 capsules were successfully fabricated by Oak Ridge National Laboratory (ORNL) and delivered to Idaho National Laboratory (INL) for irradiation in the ATR between January 2014 and October 2016. This paper describes the efforts of the team to prepare and disposition the two initial DOE-IP Co production capsules that were processed in March 2020. These efforts include performing accurate production predictions, experimentally validating predictions with assay measurements, shipping with the Orano-furnished Battelle Energy Alliance Research Reactor shipping package, and disassembling capsules at the isotope vendor site.
2012 年,先进试验堆(ATR)的一个靶件发生破裂后,国内停止了高比活度钴的生产。美国能源部(DOE)科学办公室同位素计划(IP)责成橡树岭国家实验室和爱达荷国家实验室的一个多实验室研究人员和管理人员团队重新设计放射性同位素胶囊。这项工作的目标是设计出一种比 2012 年以前的靶件更坚固、更可靠的设计。该团队成功地完成了这项任务,创建了 DOE-IP 钴(Co)生产胶囊设计。此外,橡树岭国家实验室(ORNL)成功制造了 66 个胶囊,并于 2014 年 1 月至 2016 年 10 月在 ATR 中辐照,交付给爱达荷国家实验室(INL)。本文介绍了团队为准备和处置于 2020 年 3 月处理的两个初始 DOE-IP Co 生产胶囊所做的努力。这些努力包括进行准确的生产预测、用测定测量对预测进行实验验证、使用 Orano 提供的 Battelle 能源联盟研究堆运输包装进行运输,以及在同位素供应商现场拆卸胶囊。