Lian Chao-Sheng, Si Chen, Duan Wenhui
International Laboratory for Quantum Functional Materials of Henan, School of Physics and Microelectronics, Zhengzhou University, Zhengzhou 450001, China.
School of Materials Science and Engineering, Beihang University, Beijing 100191, China.
Nano Lett. 2021 Jan 13;21(1):709-715. doi: 10.1021/acs.nanolett.0c04357. Epub 2020 Dec 30.
Layered 2M-WS is recently observed to show Majorana bound states in vortices, but its superconducting pairing mechanism remains unknown, hindering the understanding of its topological superconducting nature. Using the Migdal-Eliashberg theory and electron-phonon Wannier interpolation, we demonstrate that both bulk and bilayer 2M-WS have a single anisotropic full-gap superconducting order of s-wave symmetry. We successfully reproduce the experimental superconducting critical temperature for the bulk and predict the bilayer 2M-WS, a two-dimensional (2D) topological metal with nontrivial edge states right at the Fermi energy, to superconduct at 7 K, much higher than that in most 2D transition metal dichalcogenides (TMDs). A distinct proximity-enhanced surface superconductivity is further revealed by simulating quasiparticle density of states. This work unveils a universal electron-phonon full-gap pairing in 2M group VI TMDs and suggests a strong intrinsic surface-bulk proximity effect for 2M-WS, paving the way to engineering topological superconductivity in TMD-based nanoscale devices.
最近观察到层状2M-WS在涡旋中表现出马约拉纳束缚态,但其超导配对机制仍然未知,这阻碍了对其拓扑超导性质的理解。利用米格达尔-埃利亚什贝格理论和电子-声子万尼尔插值法,我们证明了体相和双层2M-WS都具有单一的各向异性全带隙s波对称超导序。我们成功地再现了体相的实验超导临界温度,并预测双层2M-WS(一种在费米能级处具有非平凡边缘态的二维拓扑金属)将在7 K超导,远高于大多数二维过渡金属二卤化物(TMD)。通过模拟准粒子态密度,进一步揭示了一种独特的邻近增强表面超导性。这项工作揭示了2M族VI族TMD中普遍存在的电子-声子全带隙配对,并表明2M-WS存在强烈的本征表面-体相邻近效应,为在基于TMD的纳米级器件中设计拓扑超导性铺平了道路。