SPCMIB, CNRS UMR 5068, Université de Toulouse III Paul Sabatier, 118 route de Narbonne, 31062 Toulouse cedex 9, France.
Universität Wien, Institut für Chemische Katalyse, Währinger Straße 38, 1090 Wien, Austria and University of Silesia, Institute of Chemistry, 9th Szkolna St., 40-006 Katowice, Poland.
Dalton Trans. 2021 Feb 2;50(4):1313-1323. doi: 10.1039/d0dt03577g.
Precise control over the production of carbon monoxide (CO) is essential to exploit the therapeutic potential of this molecule. The development of photoactive CO-releasing molecules (PhotoCORMs) is therefore a promising route for future clinical applications. Herein, a tricarbonyl-rhenium(i) complex (1-TPP), which incorporates a phosphine moiety as ancilliary ligand for boosting the photochemical reactivity, and a pyridyltriazole bidentate ligand with appended 2-phenylbenzoxazole moiety for the purpose of photoluminescence, was synthesized and characterized from a chemical and crystallographic point of view. Upon irradiation in the near-UV range, complex 1-TPP underwent fast photoreaction, which was monitored through changes of the UV-vis absorption and phosphorescence spectra. The photoproducts (i.e. the dicarbonyl solvento complex 2 and one CO molecule) were identified using FTIR, 1H NMR and HRMS. The results were interpreted on the basis of DFT/TD-DFT calculations. The effective photochemical release of CO associated with clear optical variations (the emitted light passed from green to orange-red) could make 1-TPP the prototype of new photochemically-active agents, potentially useful for integration in photoCORM materials.
精确控制一氧化碳 (CO) 的产生对于挖掘该分子的治疗潜力至关重要。因此,开发光活性 CO 释放分子 (PhotoCORMs) 是未来临床应用的有前途的途径。在此,合成并从化学和晶体学的角度表征了一种三羰基铼 (i) 配合物 (1-TPP),其中包含一个膦部分作为辅助配体,以提高光化学反应性,以及一个吡啶三唑双齿配体,带有附加的 2-苯基苯并恶唑部分用于光致发光。在近紫外范围内照射时,配合物 1-TPP 经历了快速光反应,通过监测 UV-vis 吸收和磷光光谱的变化来监测。使用 FTIR、1H NMR 和 HRMS 鉴定光产物(即二羰基溶剂配合物 2 和一个 CO 分子)。结果基于 DFT/TD-DFT 计算进行了解释。与明显光学变化(发射光从绿色变为橙红色)相关的有效光化学 CO 释放,可能使 1-TPP 成为新型光活性试剂的原型,这些试剂可能有助于集成在光 CORM 材料中。