Cheng Yuan, Wu Xing, Zhang Zijian, Sun Yao, Zhao Yunshan, Zhang Yingyan, Zhang Gang
Institute of High Performance Computing, A*STAR, Singapore 138632, Singapore.
Nanoscale. 2021 Jan 28;13(3):1425-1442. doi: 10.1039/d0nr06824a.
Two-dimensional (2D) materials have received tremendous attention from the research community in the past decades, because of their numerous striking physical, chemical and mechanical properties and promising potential in a wide range of applications. This field is strongly interdisciplinary, requiring efficient integration of knowledge with different insights. In this review, we summarize the up-to-date research on the thermal and mechanical properties and thermo-mechanical correlation in 2D materials, including both theoretical and experimental insight. Firstly, the mechanical properties of 2D nanomaterials are discussed, in which the underlying physics is summarized. Then, we discuss the impacts of thermal fluctuation on the mechanical properties. Next, from experimental points of view, we present the methods to introduce strain in 2D materials experimentally and the experimental tools to measure the degree of strain. Finally, we discuss the fundamental phonon and thermal properties of 2D materials, including the strain effects on phonon dispersion, phonon hydrodynamic behavior, phonon topological feature, ballistic thermal conductance and diffusive thermal conductivity. This article presents an advanced understanding of the mechanical and thermal properties of 2D materials, which provides new opportunities for promoting their applications in nanoscale electronic, optoelectronic, and thermal functional devices.
在过去几十年里,二维(2D)材料因其众多引人注目的物理、化学和机械性能以及在广泛应用中展现出的巨大潜力,受到了研究界的极大关注。该领域具有很强的跨学科性,需要将具有不同见解的知识进行有效整合。在这篇综述中,我们总结了关于二维材料热性能、机械性能以及热 - 机械相关性的最新研究,包括理论和实验方面的见解。首先,讨论了二维纳米材料的机械性能,并总结了其背后的物理原理。然后,我们探讨了热涨落对机械性能的影响。接下来,从实验角度出发,介绍了在二维材料中引入应变的实验方法以及测量应变程度的实验工具。最后,我们讨论了二维材料的基本声子和热性能,包括应变对声子色散、声子流体动力学行为、声子拓扑特征、弹道热导率和扩散热导率的影响。本文对二维材料的机械和热性能进行了深入理解,为推动其在纳米级电子、光电子和热功能器件中的应用提供了新机遇。