Richard David, Kapteijns Geert, Giannini Julia A, Manning M Lisa, Lerner Edan
Institute for Theoretical Physics, University of Amsterdam, Science Park 904, Amsterdam 1098 XH, Netherlands.
Department of Physics, Syracuse University, Syracuse, New York 13244, USA.
Phys Rev Lett. 2021 Jan 8;126(1):015501. doi: 10.1103/PhysRevLett.126.015501.
Plastic deformation in amorphous solids is known to be carried by stress-induced localized rearrangements of a few tens of particles, accompanied by the conversion of elastic energy to heat. Despite their central role in determining how glasses yield and break, the search for a simple and generally applicable definition of the precursors of those plastic rearrangements-the so-called shear transformation zones (STZs)-is still ongoing. Here we present a simple definition of STZs-based solely on the harmonic approximation of a glass's energy. We explain why and demonstrate directly that our proposed definition of plasticity carriers in amorphous solids is more broadly applicable compared to anharmonic definitions put forward previously. Finally, we offer an open-source library that analyzes low-lying STZs in computer glasses and in laboratory materials such as dense colloidal suspensions for which the harmonic approximation is accessible. Our results constitute a physically motivated methodological advancement towards characterizing mechanical disorder in glasses, and understanding how they yield.
已知非晶态固体中的塑性变形是由几十颗粒子的应力诱导局部重排所导致的,同时伴随着弹性能向热的转化。尽管这些局部重排在决定玻璃如何屈服和破裂方面起着核心作用,但对于这些塑性重排的前驱体——即所谓的剪切转变区(STZ)——寻找一个简单且普遍适用的定义的工作仍在进行中。在此,我们提出了一个基于玻璃能量的简谐近似的STZ简单定义。我们解释了原因,并直接证明,与先前提出的非简谐定义相比,我们所提出的非晶态固体中塑性载体的定义具有更广泛的适用性。最后,我们提供了一个开源库,用于分析计算机模拟玻璃以及实验室材料(如稠密胶体悬浮液,对于其简谐近似是可行的)中的低能STZ。我们的结果构成了朝着表征玻璃中的机械无序以及理解它们如何屈服的方向上基于物理原理的方法学进展。