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二维胶体玻璃中拓扑缺陷的实验识别

Experimental identification of topological defects in 2D colloidal glass.

作者信息

Vaibhav Vinay, Bera Arabinda, Liu Amelia C Y, Baggioli Matteo, Keim Peter, Zaccone Alessio

机构信息

Department of Physics "A. Pontremoli", University of Milan, via Celoria 16, 20133, Milan, Italy.

School of Physics and Astronomy, Monash University, Clayton, 3800, VIC, Australia.

出版信息

Nat Commun. 2025 Jan 2;16(1):55. doi: 10.1038/s41467-024-54857-z.

Abstract

Topological defects are singularities within a field that cannot be removed by continuous transformations. The definition of these irregularities requires an ordered reference configuration, calling into question whether they exist in disordered materials, such as glasses. However, recent work suggests that well-defined topological defects emerge in the dynamics of glasses, even if they are not evident in the static configuration. In this study, we reveal the presence of topological defects in the vibrational eigenspace of a two-dimensional experimental colloidal glass. These defects strongly correlate with the vibrational features and spatially correlate with each other and structural "soft spots", more prone to plastic flow. This work experimentally confirms the existence of topological defects in disordered systems revealing the complex interplay between topology, disorder, and dynamics.

摘要

拓扑缺陷是场中的奇点,无法通过连续变换消除。这些不规则性的定义需要一个有序的参考构型,这就引发了它们是否存在于无序材料(如玻璃)中的疑问。然而,最近的研究表明,即使在静态构型中不明显,明确的拓扑缺陷也会出现在玻璃的动力学过程中。在本研究中,我们揭示了二维实验性胶体玻璃的振动本征空间中存在拓扑缺陷。这些缺陷与振动特征密切相关,并且在空间上相互关联,还与更易发生塑性流动的结构“软点”相关。这项工作通过实验证实了无序系统中拓扑缺陷的存在,揭示了拓扑、无序和动力学之间的复杂相互作用。

https://cdn.ncbi.nlm.nih.gov/pmc/blobs/8553/11697214/9e5dd7e2feb9/41467_2024_54857_Fig1_HTML.jpg

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