Department of Electronic Materials Engineering, Kwangwoon University, Seoul 01897, Republic of Korea.
Department of Applied Chemistry, Dong-eui University, Busan 47227, Republic of Korea.
ACS Appl Mater Interfaces. 2021 Feb 3;13(4):5602-5613. doi: 10.1021/acsami.0c21097. Epub 2021 Jan 26.
Respiration monitoring and human sweat sensing have promising application prospects in personal healthcare data collection, disease diagnostics, and the effective prevention of human-to-human transmission of fatal viruses. Here, we have introduced a unique respiration monitoring and touchless sensing system based on a CsPbBr/BaTiO humidity-sensing layer operated by water-induced interfacial polarization and prepared using a facile aerosol deposition process. Based on the relationship between sensing ability and layer thickness, the sensing device with a 1.0 μm thick layer was found to exhibit optimal sensing performance, a result of its ideal microstructure. This sensor also exhibits the highest electrical signal variation at 0.5 kHz due to a substantial polarizability difference between high and low humidity. As a result, the CsPbBr/BaTiO sensing device shows the best signal variation of all types of breath-monitoring devices reported to date when used to monitor sudden changes in respiratory rates in diverse situations. Furthermore, the sensor can effectively detect sweat evaporation when placed 1 cm from the skin, including subtle changes in capacitance caused by finger area and motion, skin moisture, and contact time. This ultrasensitive sensor, with its fast response, provides a potential new sensing platform for the long-term daily monitoring of respiration and sweat evaporation.
呼吸监测和人体汗液感应在个人健康数据收集、疾病诊断以及有效预防致命病毒人际传播方面具有广阔的应用前景。在这里,我们引入了一种独特的呼吸监测和非接触式感应系统,该系统基于 CsPbBr/BaTiO 湿度感应层,通过水诱导的界面极化操作,并采用简单的气溶胶沉积工艺制备。基于感应能力与层厚的关系,发现具有 1.0 μm 厚层的感应器件表现出最佳的感应性能,这是由于其理想的微观结构。由于高低湿度之间存在显著的极化率差异,该传感器在 0.5 kHz 时表现出最高的电信号变化。因此,与迄今为止报道的所有类型的呼吸监测设备相比,CsPbBr/BaTiO 感测设备在监测各种情况下呼吸率的突然变化时表现出最佳的信号变化。此外,当距离皮肤 1 厘米时,传感器可以有效地检测汗液蒸发,包括手指区域和运动、皮肤湿度和接触时间引起的电容细微变化。这种超灵敏的传感器具有快速响应,为呼吸和汗液蒸发的长期日常监测提供了一个潜在的新传感平台。