• 文献检索
  • 文档翻译
  • 深度研究
  • 学术资讯
  • Suppr Zotero 插件Zotero 插件
  • 邀请有礼
  • 套餐&价格
  • 历史记录
应用&插件
Suppr Zotero 插件Zotero 插件浏览器插件Mac 客户端Windows 客户端微信小程序
定价
高级版会员购买积分包购买API积分包
服务
文献检索文档翻译深度研究API 文档MCP 服务
关于我们
关于 Suppr公司介绍联系我们用户协议隐私条款
关注我们

Suppr 超能文献

核心技术专利:CN118964589B侵权必究
粤ICP备2023148730 号-1Suppr @ 2026

文献检索

告别复杂PubMed语法,用中文像聊天一样搜索,搜遍4000万医学文献。AI智能推荐,让科研检索更轻松。

立即免费搜索

文件翻译

保留排版,准确专业,支持PDF/Word/PPT等文件格式,支持 12+语言互译。

免费翻译文档

深度研究

AI帮你快速写综述,25分钟生成高质量综述,智能提取关键信息,辅助科研写作。

立即免费体验

金属-半导体隧道结中的发光:等离子体激元衰变导致电子加热的直接证据。

Light Emission in Metal-Semiconductor Tunnel Junctions: Direct Evidence for Electron Heating by Plasmon Decay.

作者信息

Shalem Guy, Erez-Cohen Omer, Mahalu Diana, Bar-Joseph Israel

机构信息

Department of Condensed Matter Physics, Weizmann Institute of Science, Rehovot 7610001, Israel.

出版信息

Nano Lett. 2021 Feb 10;21(3):1282-1287. doi: 10.1021/acs.nanolett.0c03945. Epub 2021 Jan 26.

DOI:10.1021/acs.nanolett.0c03945
PMID:33497237
原文链接:https://pmc.ncbi.nlm.nih.gov/articles/PMC7883388/
Abstract

We study metal-insulator-semiconductor tunnel junctions where the metal electrode is a patterned gold layer, the insulator is a thin layer of AlO, and the semiconductor is p-type silicon. We observe light emission due to plasmon-assisted inelastic tunneling from the metal to the silicon valence band. The emission cutoff shifts to higher energies with increasing voltage, a clear signature of electrically driven plasmons. The cutoff energy exceeds the applied voltage, and a large fraction of the emission is above the threshold, ℏω > . We find that the emission spectrum manifests the Fermi-Dirac distribution of the electrons in the gold electrode. This distribution can be used to determine the effective electron temperature, , which is shown to have a linear dependence on the applied voltage. The strong correlation of with the plasmon energy serves as evidence that the mechanism for heating the electrons is plasmon decay at the source metal electrode.

摘要

我们研究了金属-绝缘体-半导体隧道结,其中金属电极是图案化的金层,绝缘体是AlO薄层,半导体是p型硅。我们观察到由于等离子体激元辅助的非弹性隧穿从金属到硅价带而产生的光发射。随着电压增加,发射截止能量向更高能量移动,这是电驱动等离子体激元的明显特征。截止能量超过施加电压,并且很大一部分发射高于阈值,ħω > 。我们发现发射光谱体现了金电极中电子的费米-狄拉克分布。这种分布可用于确定有效电子温度, ,结果表明它与施加电压呈线性关系。 与等离子体激元能量的强相关性证明了电子加热机制是源金属电极处的等离子体激元衰变。

https://cdn.ncbi.nlm.nih.gov/pmc/blobs/8645/7883388/9337d158932f/nl0c03945_0004.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/8645/7883388/2647d1b1b9fa/nl0c03945_0001.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/8645/7883388/97ed0f44b8a9/nl0c03945_0002.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/8645/7883388/4af1cad534b7/nl0c03945_0003.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/8645/7883388/9337d158932f/nl0c03945_0004.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/8645/7883388/2647d1b1b9fa/nl0c03945_0001.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/8645/7883388/97ed0f44b8a9/nl0c03945_0002.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/8645/7883388/4af1cad534b7/nl0c03945_0003.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/8645/7883388/9337d158932f/nl0c03945_0004.jpg

相似文献

1
Light Emission in Metal-Semiconductor Tunnel Junctions: Direct Evidence for Electron Heating by Plasmon Decay.金属-半导体隧道结中的发光:等离子体激元衰变导致电子加热的直接证据。
Nano Lett. 2021 Feb 10;21(3):1282-1287. doi: 10.1021/acs.nanolett.0c03945. Epub 2021 Jan 26.
2
Electrically Driven Plasmons in Metal-Insulator-Semiconductor Tunnel Junctions: The Role of Silicon Amorphization.金属-绝缘体-半导体隧道结中的电驱动等离子体:非晶硅化的作用。
Nano Lett. 2023 Mar 22;23(6):2233-2238. doi: 10.1021/acs.nanolett.2c04863. Epub 2023 Mar 1.
3
Electrically Driven Hot-Carrier Generation and Above-Threshold Light Emission in Plasmonic Tunnel Junctions.等离子体隧道结中的电驱动热载流子产生及阈值以上发光
Nano Lett. 2020 Aug 12;20(8):6067-6075. doi: 10.1021/acs.nanolett.0c02121. Epub 2020 Jun 30.
4
Plasmonic photosensitization of a wide band gap semiconductor: converting plasmons to charge carriers.宽禁带半导体的等离子体敏化:将等离子体转化为载流子。
Nano Lett. 2011 Dec 14;11(12):5548-52. doi: 10.1021/nl203457v. Epub 2011 Nov 3.
5
Electrically Driven Deterministic Plasmon Light Sources Based on Arrays of Molecular Tunnel Junctions.基于分子隧道结阵列的电驱动确定性等离子体光源。
Nano Lett. 2024 Aug 7;24(31):9720-9726. doi: 10.1021/acs.nanolett.4c02523. Epub 2024 Jul 25.
6
Tunable directional emission from electrically driven nano-strip metal-insulator-metal tunnel junctions.电驱动纳米条金属-绝缘体-金属隧道结的可调谐定向发射
Nanoscale Adv. 2022 Aug 8;4(17):3609-3616. doi: 10.1039/d2na00149g. eCollection 2022 Aug 23.
7
Ultrasmall Plasmonic Single Nanoparticle Light Source Driven by a Graphene Tunnel Junction.由石墨烯隧道结驱动的超小等离子体单纳米颗粒光源。
ACS Nano. 2018 Mar 27;12(3):2780-2788. doi: 10.1021/acsnano.7b09163. Epub 2018 Mar 14.
8
Nano-antenna enhanced waveguide integrated light source based on an MIS tunnel junction.基于金属-绝缘体-半导体(MIS)隧道结的纳米天线增强型波导集成光源。
Opt Lett. 2019 May 1;44(9):2330-2333. doi: 10.1364/OL.44.002330.
9
Upconversion electroluminescence in 2D semiconductors integrated with plasmonic tunnel junctions.与等离子体隧道结集成的二维半导体中的上转换电致发光。
Nat Nanotechnol. 2024 Jul;19(7):993-999. doi: 10.1038/s41565-024-01650-0. Epub 2024 Apr 19.
10
Enhancement of Radiative Plasmon Decay by Hot Electron Tunneling.热电子隧道增强辐射等离子体衰减。
ACS Nano. 2015 Aug 25;9(8):8176-83. doi: 10.1021/acsnano.5b02361. Epub 2015 Jul 29.

引用本文的文献

1
Light-Matter Interaction in Ultrastable Tunneling Nanogaps.超稳定隧穿纳米间隙中的光与物质相互作用
ACS Nano. 2025 Aug 5;19(30):27204-27214. doi: 10.1021/acsnano.5c03217. Epub 2025 Jul 23.
2
Molecular scale nanophotonics: hot carriers, strong coupling, and electrically driven plasmonic processes.分子尺度的纳米光子学:热载流子、强耦合和电驱动等离子体激元过程。
Nanophotonics. 2024 Mar 28;13(13):2281-2322. doi: 10.1515/nanoph-2023-0710. eCollection 2024 May.
3
Broadband Tunable Infrared Light Emission from Metal-Oxide-Semiconductor Tunnel Junctions in Silicon Photonics.

本文引用的文献

1
Electrically Driven Hot-Carrier Generation and Above-Threshold Light Emission in Plasmonic Tunnel Junctions.等离子体隧道结中的电驱动热载流子产生及阈值以上发光
Nano Lett. 2020 Aug 12;20(8):6067-6075. doi: 10.1021/acs.nanolett.0c02121. Epub 2020 Jun 30.
2
Electrically-driven Yagi-Uda antennas for light.用于光的电驱动八木-宇田天线。
Nat Commun. 2020 Jan 8;11(1):115. doi: 10.1038/s41467-019-14011-6.
3
Electrically Driven Optical Antennas Based on Template Dielectrophoretic Trapping.基于模板介电泳捕获的电驱动光学天线
硅光子学中金属氧化物半导体隧道结的宽带可调谐红外光发射
Nano Lett. 2024 Jan 24;24(3):859-865. doi: 10.1021/acs.nanolett.3c03684. Epub 2023 Dec 5.
4
Electrically Driven Plasmons in Metal-Insulator-Semiconductor Tunnel Junctions: The Role of Silicon Amorphization.金属-绝缘体-半导体隧道结中的电驱动等离子体:非晶硅化的作用。
Nano Lett. 2023 Mar 22;23(6):2233-2238. doi: 10.1021/acs.nanolett.2c04863. Epub 2023 Mar 1.
ACS Nano. 2019 Dec 24;13(12):14041-14047. doi: 10.1021/acsnano.9b06376. Epub 2019 Nov 25.
4
Antenna surface plasmon emission by inelastic tunneling.通过非弹性隧穿实现的天线表面等离子体发射。
Nat Commun. 2019 Oct 30;10(1):4949. doi: 10.1038/s41467-019-12866-3.
5
Optical antennas driven by quantum tunneling: a key issues review.由量子隧穿驱动的光学天线:关键问题综述
Rep Prog Phys. 2019 Nov;82(11):112401. doi: 10.1088/1361-6633/ab4239. Epub 2019 Sep 6.
6
Manipulation of the dephasing time by strong coupling between localized and propagating surface plasmon modes.通过局域和传播表面等离激元模式的强耦合来控制退相时间。
Nat Commun. 2018 Nov 19;9(1):4858. doi: 10.1038/s41467-018-07356-x.
7
Quantum Coherent Multielectron Processes in an Atomic Scale Contact.原子尺度接触中的量子相干多电子过程
Phys Rev Lett. 2017 Aug 11;119(6):066803. doi: 10.1103/PhysRevLett.119.066803. Epub 2017 Aug 10.
8
Fano Resonance in an Electrically Driven Plasmonic Device.电驱动等离子体器件中的法诺共振。
Nano Lett. 2016 Jan 13;16(1):748-52. doi: 10.1021/acs.nanolett.5b04622. Epub 2016 Jan 4.
9
Spontaneous Hot-Electron Light Emission from Electron-Fed Optical Antennas.电子供体光天线的自发热电子光发射。
Nano Lett. 2015 Sep 9;15(9):5811-8. doi: 10.1021/acs.nanolett.5b01861. Epub 2015 Aug 5.
10
Theory of light emission from quantum noise in plasmonic contacts: above-threshold emission from higher-order electron-plasmon scattering.等离子体接触中量子噪声产生光发射的理论:高阶电子 - 等离子体散射产生的阈上发射
Phys Rev Lett. 2015 Mar 27;114(12):126803. doi: 10.1103/PhysRevLett.114.126803. Epub 2015 Mar 26.