Kooser Kuno, Kivimäki Antti, Turunen Paavo, Pärna Rainer, Reisberg Liis, Kirm Marco, Valden Mika, Huttula Marko, Kukk Edwin
Department of Physics and Astronomy, University of Turku, FIN-20014 Turku, Finland.
Nano and Molecular Systems Research Unit, University of Oulu, PO Box 3000, FIN-90014 Oulu, Finland.
J Synchrotron Radiat. 2020 Jul 1;27(Pt 4):1080-1091. doi: 10.1107/S1600577520007146. Epub 2020 Jun 22.
Since spring 2019 an experimental setup consisting of an electron spectrometer and an ion time-of-flight mass spectrometer for diluted samples has been available for users at the FinEstBeAMS beamline of the MAX IV Laboratory in Lund, Sweden. The setup enables users to study the interaction of atoms, molecules, (molecular) microclusters and nanoparticles with short-wavelength (vacuum ultraviolet and X-ray) synchrotron radiation and to follow the electron and nuclear dynamics induced by this interaction. Test measurements of N and thiophene (CHS) molecules have demonstrated that the setup can be used for many-particle coincidence spectroscopy. The measurements of the Ar 3p photoelectron spectra by linear horizontal and vertical polarization show that angle-resolved experiments can also be performed. The possibility to compare the electron spectroscopic results of diluted samples with solid targets in the case of CoO and FeO at the Co and Fe L-absorption edges in the same experimental session is also demonstrated. Because the photon energy range of the FinEstBeAMS beamline extends from 4.4 eV up to 1000 eV, electron, ion and coincidence spectroscopy studies can be executed in a very broad photon energy range.
自2019年春季以来,瑞典隆德MAX IV实验室的FinEstBeAMS光束线为用户提供了一套由电子能谱仪和用于稀释样品的离子飞行时间质谱仪组成的实验装置。该装置使用户能够研究原子、分子、(分子)微团簇和纳米颗粒与短波长(真空紫外和X射线)同步辐射的相互作用,并追踪这种相互作用引起的电子和核动力学。对N和噻吩(CHS)分子的测试测量表明,该装置可用于多粒子符合光谱学。通过线性水平和垂直偏振对Ar 3p光电子能谱的测量表明,也可以进行角分辨实验。在同一实验环节中,还展示了在CoO和FeO的Co和Fe L吸收边处,将稀释样品与固体靶的电子能谱结果进行比较的可能性。由于FinEstBeAMS光束线的光子能量范围从4.4 eV扩展到1000 eV,因此可以在非常宽的光子能量范围内进行电子、离子和符合光谱学研究。