Valmianski Ilya, Rodríguez Arantxa Fraile, Rodríguez-Álvarez Javier, García Del Muro Montserrat, Wolowiec Christian, Kronast Florian, Ramírez Juan Gabriel, Schuller Ivan K, Labarta Amílcar, Batlle Xavier
Department of Physics and Center for Advanced Nanoscience, University of California San Diego, La Jolla, CA 92093, USA.
Departament de Física de la Matèria Condensada, Universitat de Barcelona, 08028 Barcelona, Spain and Institut de Nanociència i Nanotecnologia (IN2UB), Universitat de Barcelona, 08028 Barcelona, Spain.
Nanoscale. 2021 Mar 12;13(9):4985-4994. doi: 10.1039/d0nr08253h.
We investigate the local nanoscale changes of the magnetic anisotropy of a Ni film subject to an inverse magnetostrictive effect by proximity to a V2O3 layer. Using temperature-dependent photoemission electron microscopy (PEEM) combined with X-ray magnetic circular dichroism (XMCD), direct images of the Ni spin alignment across the first-order structural phase transition (SPT) of V2O3 were obtained. We find an abrupt temperature-driven reorientation of the Ni magnetic domains across the SPT, which is associated with a large increase of the coercive field. Moreover, angular dependent ferromagnetic resonance (FMR) shows a remarkable change in the magnetic anisotropy of the Ni film across the SPT of V2O3. Micromagnetic simulations based on these results are in quantitative agreement with the PEEM data. Direct measurements of the lateral correlation length of the Ni domains from XMCD images show an increase of almost one order of magnitude at the SPT compared to room temperature, as well as a broad spatial distribution of the local transition temperatures, thus corroborating the phase coexistence of Ni anisotropies caused by the V2O3 SPT. We show that the rearrangement of the Ni domains is due to strain induced by the oxide layers' structural domains across the SPT. Our results illustrate the use of alternative hybrid systems to manipulate magnetic domains at the nanoscale, which allows for engineering of coercive fields for novel data storage architectures.
我们研究了通过靠近V2O3层而受到逆磁致伸缩效应影响的镍薄膜磁各向异性的局部纳米尺度变化。利用温度依赖型光发射电子显微镜(PEEM)结合X射线磁圆二色性(XMCD),获得了V2O3一级结构相变(SPT)过程中镍自旋排列的直接图像。我们发现,在SPT过程中,镍磁畴会因温度驱动而突然重新取向,这与矫顽场的大幅增加有关。此外,角度相关的铁磁共振(FMR)表明,在V2O3的SPT过程中,镍薄膜的磁各向异性发生了显著变化。基于这些结果的微磁模拟与PEEM数据在定量上一致。通过XMCD图像对镍畴横向相关长度的直接测量表明,与室温相比,在SPT时该长度增加了近一个数量级,并且局部转变温度存在广泛的空间分布,从而证实了由V2O3 SPT引起的镍各向异性的相共存。我们表明,镍畴的重新排列是由于SPT过程中氧化层结构畴引起的应变所致。我们的结果说明了使用替代混合系统在纳米尺度上操纵磁畴,这有助于为新型数据存储架构设计矫顽场。