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利用硅纳米颗粒的非线性光发射映射光的磁场强度

Mapping the Magnetic Field Intensity of Light with the Nonlinear Optical Emission of a Silicon Nanoparticle.

作者信息

Li Guang-Can, Xiang Jin, Zhang Yong-Liang, Deng Fu, Panmai Mingcheng, Zhuang Weijie, Lan Sheng, Lei Dangyuan

机构信息

Guangdong Provincial Key Laboratory of Nanophotonic Functional Materials and Devices, School of Information and Optoelectronic Science and Engineering, South China Normal University, Guangzhou, 510006, China.

Department of Materials Science and Engineering, City University of Hong Kong, 83 Tat. Chee Avenue, Kowloon, Hong Kong SAR.

出版信息

Nano Lett. 2021 Mar 24;21(6):2453-2460. doi: 10.1021/acs.nanolett.0c04706. Epub 2021 Mar 2.

Abstract

To detect the magnetic component of arbitrary unknown optical fields, a candidate probe must meet a list of demanding requirements, including a spatially isotropic magnetic response, suppressed electric effect, and wide operating bandwidth. Here, we show that a silicon nanoparticle satisfies all these requirements, and its optical magnetism driven multiphoton luminescence enables direct mapping of the magnetic field intensity distribution of a tightly focused femtosecond laser beam with varied polarization orientation and spatially overlapped electric and magnetic components. Our work establishes a powerful nonlinear optics paradigm for probing unknown optical magnetic fields of arbitrary electromagnetic structures, which is not only essential for realizing subwavelength-scale optical magnetometry but also facilitates nanophotonic research in the magnetic light-matter interaction regime.

摘要

为了检测任意未知光场的磁性成分,候选探针必须满足一系列苛刻的要求,包括空间各向同性的磁响应、抑制电效应以及宽工作带宽。在此,我们表明硅纳米颗粒满足所有这些要求,并且其光学磁性驱动的多光子发光能够直接绘制具有不同偏振取向以及空间重叠的电和磁成分的紧聚焦飞秒激光束的磁场强度分布。我们的工作建立了一种强大的非线性光学范式,用于探测任意电磁结构的未知光学磁场,这不仅对于实现亚波长尺度的光磁测量至关重要,而且还促进了磁光物质相互作用领域的纳米光子学研究。

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