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[长江经济带湖北省人为源挥发性有机物排放清单及变化特征]

[VOCs Emission Inventory and Variation Characteristics of Artificial Sources in Hubei Province in the Yangtze River Economic Belt].

作者信息

Dai Ling-Wen, Meng Jing, Li Qian-Qian, Shi Bin, Su Gui-Jin, Huang Li-Hong

机构信息

College of Materials and Chemistry & Chemical Engineering, Chengdu University of Technology, Chengdu 610059, China.

Research Center for Eco-Environmental Sciences, Chinese Academy of Sciences, Beijing 100085, China.

出版信息

Huan Jing Ke Xue. 2021 Mar 8;42(3):1039-1052. doi: 10.13227/j.hjkx.202009043.

Abstract

In this study, a 2018 anthropogenic volatile organic compounds (VOCs) emission inventory in Hubei Province was conducted using the emission factor method based on activity levels of five sources. The emission characteristics and variation trends of process sources from 2009 to 2018 were further analyzed. Total anthropogenic VOCs emissions were 6.52×10 tons in Hubei Province, accounting for about 6.41% of the country's total omissions. The contributions of fossil combustion sources, process sources, solvent sources, mobile sources, and waste disposal sources were 3.26%, 76.39%, 4.54%, 14.72%, and 1.09%, respectively. Process sources involving 45 sub-categories of nine industries accounted for a significant proportion of VOCs emissions, with Wuhan and Yichang recording the highest VOCs emission levels. The VOCs emissions intensity of each city and state were analyzed based the level of economic activity and territorial area. Tianmen and Shennongjia had higher VOCs emissions per unit of GDP, while Wuhan, Ezhou, and Tianmen had higher VOCs emissions per unit area. Regarding process source contributions, VOCs emissions increased progressively to 2.45×10 tons in 2009 and then stabilized between 2015 and 2017 with maximum emissions of 7.01×10 tons. In 2018, VOCs emissions decreased to 4.98×10 tons. This trend was similar to national anthropogenic emissions. Two industrial sectors, namely chemical raw materials and rubber and plastics, were the main driving force with contributions of 33.85%-51.55% and 7.07%-38.13%, respectively. Among them, the production of chemicals and active pesticide and pharmaceutical ingredients played an important role in contributing to VOCs emissions, while emissions during foam plastics production varied greatly, increasing sharply to more than 2.00×10 tons in 2015-2017. Under the guidance of the relevant national and local policies, emissions from key industries were significantly reduced in Hubei Province.

摘要

本研究采用基于五类源活动水平的排放因子法,开展了2018年湖北省人为源挥发性有机物(VOCs)排放清单编制工作。进一步分析了2009年至2018年过程源的排放特征及变化趋势。湖北省人为源VOCs排放总量为6.52×10吨,约占全国排放总量的6.41%。化石燃烧源、过程源、溶剂源、移动源和废物处理源的贡献分别为3.26%、76.39%、4.54%、14.72%和1.09%。涉及九个行业45个子类别的过程源在VOCs排放中占比显著,武汉和宜昌的VOCs排放水平最高。基于经济活动水平和地域面积分析了各市州的VOCs排放强度。天门和神农架单位GDP的VOCs排放量较高,而武汉、鄂州和天门单位面积的VOCs排放量较高。关于过程源贡献,VOCs排放量在2009年逐渐增加至2.45×10吨,然后在2015年至2017年期间稳定下来,最大排放量为7.01×10吨。2018年,VOCs排放量降至4.98×10吨。这一趋势与全国人为排放情况相似。化学原料以及橡胶和塑料这两个工业部门是主要驱动力,贡献分别为33.85% - 51.55%和7.07% - 38.13%。其中,化学品以及活性农药和医药成分的生产对VOCs排放贡献显著,而泡沫塑料生产过程中的排放量变化很大,在2015 - 2017年急剧增加至超过2.00×10吨。在国家和地方相关政策引导下,湖北省重点行业排放量显著下降。

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