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在新冠疫情早期从太空观测到的全球甲醛(HCHO)柱浓度显著变化。

Global Significant Changes in Formaldehyde (HCHO) Columns Observed From Space at the Early Stage of the COVID-19 Pandemic.

作者信息

Sun Wenfu, Zhu Lei, De Smedt Isabelle, Bai Bin, Pu Dongchuan, Chen Yuyang, Shu Lei, Wang Dakang, Fu Tzung-May, Wang Xiaofei, Yang Xin

机构信息

School of Environmental Science and Engineering Southern University of Science and Technology Shenzhen China.

Division of Atmospheric Composition Royal Belgian Institute for Space Aeronomy (BIRA-IASB) Brussels Belgium.

出版信息

Geophys Res Lett. 2021 Feb 28;48(4):2e020GL091265. doi: 10.1029/2020GL091265. Epub 2021 Feb 23.

Abstract

Satellite HCHO data are widely used as a reliable proxy of non-methane volatile organic compounds (NMVOCs) to constrain underlying emissions and chemistry. Here, we examine global significant changes in HCHO columns at the early stage of the COVID-19 pandemic (January-April 2020) compared with the same period in 2019 with observations from the TROPOspheric Monitoring Instrument (TROPOMI). HCHO columns decline (11.0%) in the Northern China Plain (NCP) because of a combination of meteorological impacts, lower HCHO yields as NO emission plunges (by 36.0%), and reduced NMVOC emissions (by 15.0%) resulting from the lockdown. HCHO columns change near Beijing (+8.4%) due mainly to elevated hydroxyl radical as NO emission decreases in a NO -saturated regime. HCHO columns change in Australia (+17.5%), Northeastern Myanmar of Southeast Asia (+14.9%), Central Africa (+7.8%), and Central America (+18.9%), consistent with fire activities. Our work also points to other changes related to temperature and meteorological variations.

摘要

卫星甲醛数据被广泛用作非甲烷挥发性有机化合物(NMVOCs)的可靠替代指标,以限制潜在排放和化学过程。在此,我们利用对流层监测仪器(TROPOMI)的观测数据,研究了2019年同期相比,新冠疫情早期(2020年1月至4月)全球甲醛柱浓度的显著变化。由于气象影响、随着氮氧化物排放量骤降(36.0%)导致甲醛产量降低以及封锁造成的非甲烷挥发性有机化合物排放量减少(15.0%),中国北方平原(NCP)的甲醛柱浓度下降(11.0%)。北京附近的甲醛柱浓度变化(+8.4%)主要是由于在氮氧化物饱和状态下,随着氮氧化物排放量减少,羟基自由基浓度升高。澳大利亚(+17.5%)、东南亚缅甸东北部(+14.9%)、中非(+7.8%)和中美洲(+18.9%)的甲醛柱浓度变化与火灾活动一致。我们的研究还指出了与温度和气象变化相关的其他变化。

https://cdn.ncbi.nlm.nih.gov/pmc/blobs/f240/7995117/2614838912d1/GRL-48-2e020GL091265-g002.jpg

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