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碳纳米管/二硫化钨可见光谱光电探测器的制备

Fabrication of a carbon nanotube/tungsten disulfide visible spectrum photodetector.

作者信息

Rashid Haroon, Sapiee Nurfarhana Mohamad, Arsad Norhana, Ahmad Harith, Bakar Ahmad Ashrif A, Reaz Mamun Ibne

出版信息

Appl Opt. 2021 Apr 1;60(10):2839-2845. doi: 10.1364/AO.417230.

DOI:10.1364/AO.417230
PMID:33798162
Abstract

Two-dimensional-material-based photodetectors are gaining prominence in optoelectronic applications, but there are certain factors to consider with bulk material usage. The demand for a highly responsive and highly efficient device with an inexpensive fabrication method is always of paramount importance. Carbon nanotubes (CNT) are well known, owing to their upheld vigorous structural and optoelectronic characteristics, but to fabricate them at a large scale involves multifarious processes. A visible range photodetector device structure developed using a simple and inexpensive drop-casting technique is reported here. The optoelectronic characteristics of the device are studied with IV measurements under the light and dark conditions by incorporating a thin CNT layer on top of tungsten-disulfide-based heterojunction photodetector to enhance the overall characteristics such as detectivity, responsivity, photocurrent, rise time, and fall time in the visible range of the light spectrum with a violet light source at 441 nm. In the DC bias voltage range of -20 to 20 V, IV measurements are carried out under dark and illumination conditions with different incident power densities. The threshold voltage is recognized at 2.0 V. Photocurrent is found to be highly dependent on the state of the incident light. For 0.3074/ illuminated power, the highest responsivity and detectivity are determined to be 0.57 A/W and 2.89×10 Jones. These findings encourage an alternative fabrication method at a large scale to grow CNTs for the enhancement of optoelectronic properties of present two-dimensional-material-based optoelectronic and photonics applications.

摘要

基于二维材料的光电探测器在光电子应用中日益突出,但在使用块状材料时需要考虑某些因素。对于具有廉价制造方法的高响应性和高效器件的需求始终至关重要。碳纳米管(CNT)因其保持的强大结构和光电特性而广为人知,但大规模制造它们涉及多种工艺。本文报道了一种使用简单且廉价的滴铸技术开发的可见光谱范围光电探测器器件结构。通过在基于二硫化钨的异质结光电探测器顶部并入一层薄的碳纳米管层,在明暗条件下通过IV测量研究了该器件的光电特性,以增强在441nm紫光光源的可见光谱范围内的整体特性,如探测率、响应度、光电流、上升时间和下降时间。在-20至20V的直流偏置电压范围内,在不同入射功率密度的暗态和光照条件下进行IV测量。阈值电压确定为2.0V。发现光电流高度依赖于入射光的状态。对于0.3074/的光照功率,最高响应度和探测率分别确定为0.57A/W和2.89×10琼斯。这些发现鼓励大规模采用另一种制造方法来生长碳纳米管,以增强当前基于二维材料的光电子和光子学应用的光电性能。

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