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碱/锌激活粉煤灰纳米复合材料在染料去除和抗菌方面的应用。

Alkali/zinc-activated fly ash nanocomposites for dye removal and antibacterial applications.

机构信息

Civil and Environmental Engineering, Konkuk University, 120 Neungdong-ro, Gwangjin-gu, Seoul 05029, South Korea.

Department of Biotechnology, College of Life Sciences and Biotechnology, Korea University, 145 Anam-ro, Seongbuk-gu, Seoul 02841, South Korea.

出版信息

Bioresour Technol. 2021 Jul;331:125060. doi: 10.1016/j.biortech.2021.125060. Epub 2021 Mar 27.

Abstract

Fly ash (FA), obtained as waste materials from industrial power plants, is generated in large quantities and low recycling. In this study, re-generation of waste FA as cost-effective materials with adsorbent and antibacterial applications was assessed. Alkaline/zinc-activated fly ash nanocomposite (A-FA/Zn) was prepared using one-pot hydrothermal technique. Those nanocomposites are characterized by high surface area and negatively surface charge, which are important influences contributing to an enhancement in adsorption capacity via increase in the number of adsorptive sites and electrostatic interaction between dye molecules-nanocomposites. Additionally, the presence of Zn ions in the prepared nanocomposites represents a key advantage with respect to enhancing antibacterial activity. The feasibility of further enhancing adsorption and antibacterial mechanisms was also examined. It is anticipated that the findings of this study will provide useful information with respect to the development of simple, eco-friendly and low-cost A-FA/Zn with multifunctional applications as organic dye removal and antibacterial purposes.

摘要

粉煤灰(FA)是工业发电厂的废弃物,产生量大且回收利用率低。本研究评估了将废 FA 再生成具有吸附剂和抗菌应用的经济型材料。采用一锅水热技术制备了碱性/锌激活粉煤灰纳米复合材料(A-FA/Zn)。这些纳米复合材料具有高表面积和负表面电荷的特点,这是通过增加吸附位点的数量和染料分子-纳米复合材料之间的静电相互作用来提高吸附能力的重要影响因素。此外,制备的纳米复合材料中存在 Zn 离子是提高抗菌活性的一个关键优势。还研究了进一步增强吸附和抗菌机制的可行性。预计本研究的结果将为开发简单、环保且低成本的 A-FA/Zn 提供有用信息,该材料具有去除有机染料和抗菌等多种功能。

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