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稀金属ZrTe₅和HfTe₅中由热力学诱导的输运异常

Thermodynamically Induced Transport Anomaly in Dilute Metals ZrTe_{5} and HfTe_{5}.

作者信息

Wang Chenjie

机构信息

Department of Physics and HKU-UCAS Joint Institute for Theoretical and Computational Physics, The University of Hong Kong, Pokfulam Road, Hong Kong, China.

出版信息

Phys Rev Lett. 2021 Mar 26;126(12):126601. doi: 10.1103/PhysRevLett.126.126601.

Abstract

A 40-year-old puzzle in transition metal pentatellurides ZrTe_{5} and HfTe_{5} is the anomalous peak in the temperature dependence of the longitudinal resistivity, which is accompanied by sign reverses of the Hall and Seebeck coefficients. We give a plausible explanation for these phenomena without assuming any phase transition or strong interaction effect. We show that, due to intrinsic thermodynamics and diluteness of the conducting electrons in these materials, the chemical potential displays a strong dependence on the temperature and magnetic field. With that, we compute resistivity, Hall and Seebeck coefficients in zero field, and magnetoresistivity and Hall resistivity in finite magnetic fields, in all of which we reproduce the main features that are observed in experiments.

摘要

过渡金属五碲化物ZrTe₅和HfTe₅中一个存在了40年的谜题是纵向电阻率随温度变化的反常峰值,同时伴有霍尔系数和塞贝克系数的符号反转。我们在不假设任何相变或强相互作用效应的情况下,对这些现象给出了一个合理的解释。我们表明,由于这些材料中导电电子的本征热力学性质和稀释性,化学势对温度和磁场表现出强烈的依赖性。据此,我们计算了零场下的电阻率、霍尔系数和塞贝克系数,以及有限磁场下的磁阻率和霍尔电阻率,所有这些计算结果都再现了实验中观察到的主要特征。

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