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通过附着衍射皱纹图案制备高性能蓝色量子发光二极管。

High performance blue quantum light-emitting diodes by attaching diffraction wrinkle patterns.

作者信息

Qi Hui, Wang Shujie, Li Chenguang, Zhao Yaolong, Xu Bo, Jiang Xiaohong, Fang Yan, Wang Aqiang, Shen Huaibin, Du Zuliang

机构信息

Key Laboratory for Special Functional Materials of Ministry of Education, National & Local Joint Engineering Research Centre for High-efficiency Display and Lighting Technology, School of Materials and Engineering, Collaborative Innovation Centre of Nano Functional Materials and Applications, Henan University, Kaifeng 475004, China.

出版信息

Nanoscale. 2021 May 13;13(18):8498-8505. doi: 10.1039/d1nr00082a.

Abstract

Highly efficient blue quantum-dot light-emitting diodes (QLEDs) are still challenging to use in displays and solid-state lighting. Enhancing light outcoupling is one of the most effective methods to improve the performance of blue QLEDs. Here, a strategy for a spectrally independent boost in light outcoupling of blue QLEDs is demonstrated by quasi-periodic wrinkles, which are successfully used as a diffraction grating for extracting trapped light at the substrate/air interface. The quasi-periodic wrinkles can be adjusted from nano-scale to micron-scale under the condition of a constant aspect ratio, and the optimized wrinkle device shows a maximum luminance of 11 769 cd m-2 and a peak EQE of 15.41%. The enhancement of EQE is 49.5% higher compared to that of the reference device. Furthermore, simulation and calculation also indicate that external micron-scattering wrinkle patterns are an attractive option for boosting the performances of blue QLEDs.

摘要

高效蓝色量子点发光二极管(QLED)在显示器和固态照明中的应用仍然具有挑战性。提高光出射耦合是提高蓝色QLED性能的最有效方法之一。在此,通过准周期皱纹展示了一种在光谱上独立增强蓝色QLED光出射耦合的策略,这些皱纹成功地用作衍射光栅,用于提取在衬底/空气界面处被困的光。在恒定纵横比的条件下,准周期皱纹可以从纳米尺度调整到微米尺度,优化后的皱纹器件显示出最大亮度为11769 cd m-2,峰值外量子效率(EQE)为15.41%。与参考器件相比,EQE的提高高出49.5%。此外,模拟和计算还表明,外部微米级散射皱纹图案是提高蓝色QLED性能的一个有吸引力的选择。

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