Wang Xinyu, Li Fengxiang, Hu Xiaomin, Hua Tao
Department of Environmental Engineering, School of Resource and Civil Engineering, Northeastern University, Shenyang 110819, China; College of Environmental Science and Engineering, Ministry of Education Key Laboratory of Pollution Processes and Environmental Criteria, Remediation and Pollution Control for Urban Ecological Environmental, Nankai University, Tianjin 300350, China.
College of Environmental Science and Engineering, Ministry of Education Key Laboratory of Pollution Processes and Environmental Criteria, Remediation and Pollution Control for Urban Ecological Environmental, Nankai University, Tianjin 300350, China.
Sci Total Environ. 2021 Aug 25;784:146912. doi: 10.1016/j.scitotenv.2021.146912. Epub 2021 Apr 6.
Antibiotic pollution is mainly caused by aquaculture wastewater and pharmaceuticals, which are frequently used by humans. Due to limited treatment efficiency or improper selection of treatment methods, these antibiotic residues may be very harmful in human drinking water and aquatic environments. The EAOPs coupling membrane technology (EAOPs-membrane) can play their own advantages, which can significantly improve the degradation efficiency and alleviate membrane pollution (electrochemical manners). In this context, this review mainly collecting researches and information on EAOPs-membrane treatment of antibiotic pollution published between 2012 and 2020. Discussed the different combinations of these two technologies, the mechanism of them in the system to improve the processing efficiency, prolong the working time, and stabilize the system structure. Mainly due to the synergistic effect of electrochemical behavior such as electric repulsion and in-situ oxidation, the membrane fouling in the system is alleviated. In this review it was summarized that the selection of different membrane electrode materials and their modifications. The paper also elaborates the existing challenges facing the EAOPs-membrane methods for antibiotic pollution treatment, and their prospects.
抗生素污染主要由水产养殖废水和人类频繁使用的药物引起。由于处理效率有限或处理方法选择不当，这些抗生素残留可能在人类饮用水和水生环境中非常有害。电催化高级氧化工艺耦合膜技术（EAOPs-膜）可以发挥自身优势，显著提高降解效率并减轻膜污染（电化学方式）。在此背景下，本综述主要收集了2012年至2020年间发表的关于EAOPs-膜处理抗生素污染的研究和信息。讨论了这两种技术的不同组合、它们在系统中提高处理效率、延长工作时间和稳定系统结构的机制。主要由于电排斥和原位氧化等电化学行为的协同作用，系统中的膜污染得到了缓解。本综述总结了不同膜电极材料的选择及其改性。本文还阐述了EAOPs-膜方法处理抗生素污染面临的现有挑战及其前景。
