Recent Progress on Addressing the Key Challenges in Organic Thermoelectrics.

Compared with inorganic thermoelectric materials, organic thermoelectric (OTE) materials have attracted increasing attention due to their advantages of low toxicity, high mechanical flexibility, and large-scale solution processability. In the past few years, OTE materials have made remarkable progress in terms of their design, synthesis, and device performance. However, some challenges remain, including the low doping efficiency in n-type materials, poor doping stability with molecular dopants, and the largely reduced Seebeck coefficient after heavily doping, etc. All these factors hinder the further development of OTEs for commercial applications. In this Minireview, we highlight several key challenges during the development of OTEs and summarize recent understandings and efforts to address these challenges.