Technische Universität Kaiserslautern, Fachbereich Chemie - Organische Chemie, Erwin-Schrödinger-Straße 54, 67663 Kaiserslautern, Germany.
INM - Leibniz Institute for New Materials, Campus D2 2, 66123 Saarbrücken, Germany.
Org Biomol Chem. 2021 May 5;19(17):3893-3900. doi: 10.1039/d1ob00341k.
Mixed monolayer-protected gold nanoparticles containing surface-bound triethylene glycol and dipicolylamine groups aggregated in water/methanol, 1 : 2 (v/v) in the presence of nucleotides, if the solution also contained zinc(ii) nitrate to convert the dipicolylamine units into the corresponding zinc complexes. Nanoparticle aggregation could be followed with the naked eye by the colour change of the solution from red to purple followed by nanoparticle precipitation. The sensitivity was highest for adenosine triphosphate (ATP), which could be detected at concentrations >10 μM, and decreased over adenosine diphosphate (ADP) to adenosine monophosphate (AMP), consistent with the typically higher affinity of zinc(ii)-dipicolylamine-derived receptors for higher charged nucleotides. Inorganic sodium diphosphate and triphosphate interfered in the assay by also inducing nanoparticle aggregation. However, while the nucleotide-induced aggregates persisted even at higher analyte concentrations, the nanoparticles that were precipitated with inorganic salts redissolved again when the salt concentration was increased. The thus resulting solutions retained their ability to respond to nucleotides, but they now preferentially responded to AMP. Accordingly, AMP could be sensed selectively at concentrations ≥50 μM in an aqueous environment, even in the presence of other nucleotides and inorganic anions. This work thus introduces a novel approach for the sensing of a nucleotide that is often the most difficult analyte to detect with other assays.
混合单层保护的金纳米粒子含有表面结合的三乙二醇和二吡啶胺基团,如果溶液中还含有硝酸锌(ii)以将二吡啶胺单元转化为相应的锌配合物,则在水/甲醇(1:2,v/v)中聚集。如果溶液中还含有硝酸锌(ii)以将二吡啶胺单元转化为相应的锌配合物,则可以通过肉眼观察到纳米粒子的聚集,溶液的颜色从红色变为紫色,随后是纳米粒子的沉淀。对于三磷酸腺苷(ATP),灵敏度最高,可在浓度>10 μM 时检测到,对于二磷酸腺苷(ADP)和一磷酸腺苷(AMP)则降低,这与锌(ii)-二吡啶胺衍生受体通常对带更高电荷的核苷酸具有更高亲和力的情况一致。无机磷酸二钠和三磷酸钠通过诱导纳米粒子聚集也会干扰测定。然而,尽管与无机盐沉淀的纳米粒子在更高分析物浓度下仍然存在,但当盐浓度增加时,它们又重新溶解。因此,即使在存在其他核苷酸和无机阴离子的情况下,该溶液仍保留其对核苷酸的响应能力,但现在优先响应 AMP。因此,即使在水溶液中,AMP 也可以在浓度≥50 μM 时被选择性地检测到,即使存在其他核苷酸和无机阴离子也是如此。这项工作因此引入了一种新的方法来检测通常是其他测定方法最难检测的分析物——核苷酸。