State Environmental Protection Key Laboratory of Urban Ambient Air Particulate Matter Pollution Prevention and Control, College of Environmental Science and Engineering, Nankai University, Tianjin, 300350, China; CMA-NKU Cooperative Laboratory for Atmospheric Environment-Health Research (CLAER), College of Environmental Science and Engineering, Nankai University, Tianjin, 300350, China.
CMA-NKU Cooperative Laboratory for Atmospheric Environment-Health Research (CLAER), College of Environmental Science and Engineering, Nankai University, Tianjin, 300350, China; Tianjin Environmental Meteorological Center, Tianjin, 300074, China.
Environ Pollut. 2021 Oct 1;286:117252. doi: 10.1016/j.envpol.2021.117252. Epub 2021 May 6.
Potential health benefits from improved ambient air quality during the COVID-19 shutdown have been recently reported and discussed. Despite the shutdown measures being in place, northern China still suffered severe haze episodes (HE) that are not yet fully understood, particularly how the source emissions changed. Thus, the meteorological conditions and source emissions in processing five HEs occurred in Beijing-Tianjin-Hebei area were investigated by analyzing a comprehensive real-time measurement dataset including air quality data, particle physics, optical properties, chemistry, aerosol lidar remote sensing, and meteorology. Three HEs recorded before the shutdown began were related to accumulated primary pollutants and secondary aerosol formation under unfavorable dispersion conditions. The common "business as usual" emissions from local primary sources in this highly polluted area exceeded the wintertime atmospheric diffusive capacity to disperse them. Thus, an intensive haze formed under these adverse meteorological conditions such as in the first HE, with coal combustion to be the predominant source. Positive responses to the shutdown measures were demonstrated by reduced contributions from traffic and dust during the final two HEs that overlapped the Spring and Lantern Festivals, respectively. Local meteorological dispersion during the Spring Festival was the poorest among the five HEs. Increased residential burning plus fireworks emissions contributed to the elevated PM with the potential of enhancing the HEs. Our results highlight that reductions from shutdown measures alone do not prevent the occurrence of HEs. To further reduce air pollution and thus improve public health, abatement strategies with an emphasis on residential burning are needed.
最近有报道称,改善 COVID-19 封锁期间的环境空气质量可能会带来健康益处,并对此进行了讨论。尽管采取了封锁措施,但中国北方仍遭受了严重的雾霾事件(HE),这些事件尚未得到充分理解,特别是源排放的变化情况。因此,通过分析包括空气质量数据、颗粒物理、光学特性、化学、气溶胶激光雷达遥感和气象在内的综合实时测量数据集,研究了京津冀地区发生的五次 HE 期间的气象条件和源排放情况。在封锁开始之前记录的三次 HE 与不利扩散条件下积累的一次污染物和二次气溶胶形成有关。在这个污染严重的地区,来自当地一次源的常见“照常营业”排放超过了冬季大气的扩散能力,无法将其驱散。因此,在这些不利的气象条件下形成了强烈的雾霾,第一次 HE 中以煤炭燃烧为主导源。在最后两次 HE 期间,恰逢春节和元宵节,交通和扬尘的贡献分别减少,表明对封锁措施的积极响应。春节期间的当地气象扩散是五次 HE 中最差的。居民燃烧加上烟花排放的增加导致 PM 升高,有可能加剧 HE。我们的研究结果表明,仅靠封锁措施并不能防止 HE 的发生。为了进一步减少空气污染,改善公众健康,需要采取以居民燃烧为重点的减排策略。