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临汾市汾渭平原 COVID-19 前后空气污染来源变化及其对健康影响

Variation of pollution sources and health effects on air pollution before and during COVID-19 pandemic in Linfen, Fenwei Plain.

机构信息

School of Environmental Studies & State Key Laboratory of Biogeology and Environmental Geology, China University of Geosciences, Wuhan, 430074, China; Hubei Key Laboratory of Mine Environmental Pollution Control and Remediation, School of Environmental Science and Engineering, Hubei Polytechnic University, Huangshi, 435003, China.

School of Environmental Studies & State Key Laboratory of Biogeology and Environmental Geology, China University of Geosciences, Wuhan, 430074, China.

出版信息

Environ Res. 2022 Oct;213:113719. doi: 10.1016/j.envres.2022.113719. Epub 2022 Jun 24.

Abstract

Stringent pollution control measures are generally applied to improve air quality, especially in the Spring Festival in China. Meanwhile, human activities are reduced significantly due to nationwide lockdown measures to curtail the COVID-19 spreading in 2020. Herein, to better understand the influence of control measures and meteorology on air pollution, this study compared the variation of pollution source and their health risk during the 2019 and 2020 Spring Festival in Linfen, China. Results revealed that the average concentration of PM in 2020 decreased by 39.0% when compared to the 2019 Spring Festival. Organic carbon (OC) and SO were the primary contributor to PM with the value of 19.5% (21.1%) and 23.5% (25.5%) in 2019 (2020) Spring Festival, respectively. Based on the positive matrix factorization (PMF) model, six pollution sources of PM were indicated. Vehicle emissions (VE) had the maximum reduction in pollution source concentration (28.39 μg· m), followed by dust fall (DF) (11.47 μg· m), firework burning (FB) (10.39 μg· m), coal combustion (CC) (8.54 μg· m), and secondary inorganic aerosol (SIA) (3.95 μg· m). However, the apportionment concentration of biomass burning (BB) increased by 78.7%, indicating a significant increase in biomass combustion under control measures. PAHs-lifetime lung cancer risk (ILCR) of VE, CC, FB, BB, and DF, decreased by 44.6%, 43.2%, 34.1%, 21.3%, and 2.0%, respectively. Additionally, the average contribution of meteorological conditions on PM in 2020 increased by 20.21% compared to 2019 Spring Festival, demonstrating that meteorological conditions played a crucial role in located air pollution. This study revealed that the existing control measures in Linfen were efficient to reduce air pollution and health risk, whereas more BB emissions were worthy of further attention. Furthermore, the result was conducive to developing more effective control measures and putting more attention into unfavorable meteorological conditions in Linfen.

摘要

在中国,通常会采取严格的污染控制措施来改善空气质量,尤其是在春节期间。同时,由于 2020 年全国范围内采取了封锁措施以遏制 COVID-19 的传播,人类活动也大幅减少。在此背景下,为了更好地了解控制措施和气象条件对空气污染的影响,本研究比较了中国临汾市 2019 年和 2020 年春节期间污染源的变化及其对健康的风险。结果表明,与 2019 年春节相比,2020 年春节期间 PM 的平均浓度下降了 39.0%。在 PM 中,有机碳(OC)和 SO 是主要贡献者,其值分别为 19.5%(2019 年春节)和 23.5%(2020 年春节)。基于正定矩阵因子(PMF)模型,指出了 PM 的六个污染源。车辆排放(VE)的污染源浓度降幅最大(28.39μg·m),其次是扬尘(DF)(11.47μg·m)、烟花燃烧(FB)(10.39μg·m)、煤炭燃烧(CC)(8.54μg·m)和二次无机气溶胶(SIA)(3.95μg·m)。然而,生物质燃烧(BB)的分配浓度增加了 78.7%,表明在控制措施下生物质燃烧显著增加。VE、CC、FB、BB 和 DF 的多环芳烃终生肺癌风险(ILCR)分别降低了 44.6%、43.2%、34.1%、21.3%和 2.0%。此外,与 2019 年春节相比,2020 年春节期间气象条件对 PM 的平均贡献增加了 20.21%,表明气象条件在局地空气污染中起着至关重要的作用。本研究表明,临汾市现有的控制措施能够有效降低空气污染和健康风险,而更多的 BB 排放值得进一步关注。此外,该结果有利于在临汾制定更有效的控制措施,并更加关注不利的气象条件。

https://cdn.ncbi.nlm.nih.gov/pmc/blobs/31a2/9225942/db647faf2f57/gr1_lrg.jpg

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